Observation of polaritonic flat-band bound states in the continuum in a 2D magnet

Abstract: Flat-band bound states in the continuum (BICs) are topological states with suppressed group velocity and robustness against radiation loss, offering a powerful platform for the exploration of non-Hermitian, nonlinear, topological phenomena and device applications. Van der Waals (vdW) metasurfaces have recently emerged as promising candidates for sustaining BICs and hybridizing with material transitions. However, the realization of flat-band BICs remains elusive. Here, we experimentally demonstrate polaritonic high-order BICs on a wide-angle flat band utilizing a subwavelength metasurface made of a vdW magnet CrSBr. The large oscillator strength of direct excitons in CrSBr enables near ultrastrong coupling with BICs, leading to strongly suppressed polaritonic angular dispersions. Remarkably, second-order polaritonic BICs become flat-band across a wide angular range, with corresponding Q factors exceeding 1500. Additionally, we find that these polaritonic BICs vanish in the transverse magnetic configuration, while leading to fascinating surface hyperbolic exciton-polaritons within the Reststrahlen band. Our findings underscore CrSBr as an exceptional platform for exploring flat-band photonics and polaritonics, paving the new avenue for advances in next-generation optical and quantum technologies.