Multiphoton quantum sensing (2405.16793v2)

Abstract: While the fundamental principles of light-matter interaction are well-understood and drive countless technologies, the world of multiphoton processes remains a fascinating puzzle, holding the potential to drastically alter our understanding of how light interacts with matter at its most basic level. This rich interplay of light and matter unveils novel phenomena that can be harnessed for sensing with exceptional precision, as exemplified by multiphoton quantum sensing. This thesis delves into the applications of multiphoton quantum protocols, particularly in imaging, communication, and plasmonic sensing, to surpass classical limitations and achieve enhanced sensitivity. We explore the potential of multiphoton quantum processes, particularly in the nanoscale regime and within subsystems of macroscopic systems, where novel and ultra-sensitive sensing methodologies emerge. Subsequent chapters of this thesis demonstrate the transformative potential of multiphoton quantum sensing, elucidating the design, implementation, and experimental results of specific sensing protocols tailored to diverse applications. Our analysis combines experimental observations and theoretical predictions to assess the sensitivity and performance of these protocols. Additionally, the thesis discusses potential future directions and advancements in the field, envisioning applications in biomolecule detection, environmental monitoring, and fundamental studies of light-matter interactions at the nanoscale. Concluding reflections highlight the implications of multiphoton quantum sensing across scientific disciplines and lay the groundwork for future research endeavors.