Thermal and electric field driven breakdown precursor formation on metal surfaces

Abstract: The phenomenon of electric breakdown poses serious challenge to the design of devices that operate under high gradient environments. Experimental evidence often points towards breakdown events that are accompanied by elevated temperatures and dark current spikes, presumably due to high-asperity nano-structure formation that enhances the local electric field and triggers a runaway process. However, the exact mechanistic origin of such nano-structures under typical macroscopic operational conditions of electric gradient and magnetic-field-mediated heating remains poorly understood. In this work, a model is presented that describes the evolution of a typical copper surface under the combined action of the electric fields and elevated temperatures. Using a mesoscale curvature-driven growth model, we show how the copper surface can undergo a type of dynamical instability that naturally leads to the formation of sharp asperities in realistic experimental conditions. Exploring the combined effect of fields and temperature rise, we identify critical regimes that allow for the formation of breakdown precursors. These regimes strongly resonate with previous experimental findings on breakdown of copper electrodes, hence suggesting surface diffusion to be a crucial breakdown precursor mechanism.