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$μ^+$ Knight Shift in UTe$_2$: Evidence for Relocalization in a Kondo Lattice

Published 21 Apr 2023 in cond-mat.str-el and cond-mat.supr-con | (2304.11242v1)

Abstract: The local magnetic susceptibility of the spin-triplet superconductor UTe$2$ has been investigated by positive muon ($\mu+$) Knight shift measurements in the normal state. Three distinct $\mu+$ Knight shift components are observed for a magnetic field applied parallel to the $c$ axis. Two of these exhibit a breakdown in the linear relationship with the bulk magnetic susceptibility ($\chi$) below a temperature $T* ! \sim ! 30$ K, which points to a gradual emergence of a correlated Kondo liquid. Below $T{\rm r} ! \sim ! 12$ K linearity is gradually restored, indicating partial relocalization of the Kondo liquid quasiparticles. The third Knight shift component is two orders of magnitude larger, and despite the $c$-axis alignment of the external field, scales with the $a$-axis $\chi$ above $T_{\rm r} ! \sim ! 12$ K. We conjecture that this component is associated with magnetic clusters and the change in the temperature dependence of all three Knight shift components below $T_{\rm r}$ is associated with a change in magnetic correlations. Our findings indicate that prior to the onset of superconductivity the development of the itinerant heavy-electron fluid is halted by a gradual development of local U $5f$-moment fluctuations.

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