Nonlinear optical response spatial self-hase modulation in MoTe2: correlations between \c{hi}(3) and mobility or effective mass

Abstract: We report an unambiguous observation of third-order nonlinear optical effect, spatial self-phase modulation (SSPM), in a MoTe2 dispersion. The values of the third order nonlinear optical coefficients effectively for one layer MoTe2, \c{hi}(3)one-layer, are obtained through the SSPM method at excitation wavelengths 473, 532, 750 and 801 nm, respectively. The wind-chime model is used to explain the ring formation time. The wavelength dependence of \c{hi}(3)one-layer compares well with the photo-absorption spectra. Significantly, we find a correlation between \c{hi}(3) and the carrier mobility {\mu} or effective mass m*, which again further supports the laser-induced ac electron coherence in 2D materials.