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A crossover in spatio-temporal correlations of strain fluctuations in glass forming liquids (1907.02794v2)

Published 5 Jul 2019 in cond-mat.soft and cond-mat.stat-mech

Abstract: Via molecular dynamics simulations of a generic glass former in the supercooled and normal liquid states, it is shown that spatial correlations of strain fluctuations exhibit a crossover from the well-established power-law $\sim 1/r3$-decay at long wavelengths to an exponential behavior, $\sim \exp(-r/l_{\text {c}})$ at intermediate distances. The characteristic length of the exponential decay grows both with temperature and time via, $l_{\text {c}}2 \propto D(T)\, t$, with $D(T)$ being the temperature-dependent diffusion coefficient. This suggests that the crossover between the power-law and exponential decays is governed by a diffusion process.

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