Optically trapped Feshbach molecules of fermionic 161Dy and 40K (2304.07921v2)

Abstract: We report on the preparation of a pure ultracold sample of bosonic DyK Feshbach molecules, which are composed of the fermionic isotopes 161Dy and 40K. Employing a magnetic sweep across a resonance located near 7.3 G, we produce up to 5000 molecules at a temperature of about 50 nK. For purification from the remaining atoms, we apply a Stern-Gerlach technique based on magnetic levitation of the molecules in a very weak optical dipole trap. With the trapped molecules we finally reach a high phase-space density of about 0.1. We measure the magnetic field dependence of the molecular binding energy and the magnetic moment, refining our knowledge of the resonance parameters. We also demonstrate a peculiar anisotropic expansion effect observed when the molecules are released from the trap and expand freely in the magnetic levitation field. Moreover, we identify an important lifetime limitation that is imposed by the 1064-nm infrared trap light itself and not by inelastic collisions. The light-induced decay rate is found to be proportional to the trap light intensity and the closed-channel fraction of the Feshbach molecule. These observations suggest a one-photon coupling to electronically excited states to limit the lifetime and point to the prospect of loss suppression by optimizing the wavelength of the trapping light. Our results represent important insights and experimental steps on the way to achieve quantum-degenerate samples of DyK molecules and novel superfluids based on mass-imbalanced fermion mixtures.