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Bridging ambient- and high-pressure superconductivity in La2_2LnNi2_2O7_7 films

Published 18 Aug 2026 in cond-mat.supr-con, cond-mat.mtrl-sci, and cond-mat.str-el | (2608.17745v1)

Abstract: The discovery of high critical-temperature TcT_{\mathrm{c}} superconductivity near 80 K in bilayer nickelates under high pressure has sparked extensive studies. While superconductivity exceeding 40 K was subsequently discovered at ambient pressure in compressively strained films, the relationship between ambient- and high-pressure regimes remains an open question. Here we present a systematic investigation of superconductivity in compressively strained La<em>2<em>2LnNi2_2O7_7 films (Ln = lanthanides) at ambient and high pressures. The normal-state resistivity at ambient pressure, revealed by suppressing superconductivity with magnetic fields of 59 T, tends toward T<sup>2T<sup>2 behaviour. Under high pressure in a cubic-anvil cell, T</em>cT</em>{\mathrm{c}} was enhanced from 41-42 K at ambient pressure to 67-73 K at 16 GPa. On the other hand, lattice compression induced by Ln substitution, which may mimic effects of pressure, lowers TcT_{\mathrm{c}}. In both cases, TcT_{\mathrm{c}} correlates with the evolution of normal-state transport between T<sup>2T<sup>2 and TT-linear behaviour, offering insight into the interplay between lattice structure and superconductivity in bilayer nickelates.

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