Sub-8-nm resolution AKB-mirror-based hard X-ray ptychography via generalized Wirtinger projections

Abstract: Hard X-ray ptychography has become increasingly essential in both the life and physical sciences. However, pushing resolution down to a few nanometres often requires highly customized, chromatic diffractive or refractive X-ray nanofocusing optics, significantly limiting the practical broadband energy-scan applications. Here, we present the first known hard X-ray ptychographic imaging with a half-pitch resolution below 8 nm using total-reflection Advanced Kirkpatrick-Baez (AKB) mirror nanofocusing optics at the high energy photon source (HEPS), with clear potential for further extension. Despite leveraging the benefits of enhanced instrumentation, such as the high coherent flux of 4th-generation diffraction-limited storage rings (DLSR), state-of-the-art beamline X-ray optics and detectors, this is made possible by developing a reconstruction algorithm termed Generalized Wirtinger Projections (GWP). We derive the theory of GWP and experimentally demonstrate its capability for improved partial-coherence reconstruction and enhanced spatial resolution over conventional methods through imaging experiments on a Siemens star test chart at 12.4 keV. GWP provides a highly compact framework for jointly accounting for multiple coupled uncertainties that degrade resolution, enabling straightforward extension to other imaging modalities, such as burst ptychography, while delivering nearly an order-of-magnitude improvement in GPU memory efficiency. Furthermore, the ability to combine nanometre-scale spatial resolution with the inherently achromatic nanofocusing optics demonstrated in this work potentially opens new opportunities for in situ or operando broadband, energy-scan 3D spectroscopic imaging with element- or chemical-state specificity in complex environments at the nanoscale, holding significant promise for a wide range of applications from electronics and energy science to neuroscience.