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Quenching of Nonrelativistic p-Wave Spin Splitting by c-f Decoupling in CeNiAsO

Published 1 Jun 2026 in cond-mat.str-el and cond-mat.mtrl-sci | (2606.02420v1)

Abstract: The extending of spin-space group symmetries to coplanar antiferromagnets has predicted the emergence of odd-parity nonrelativistic spin splittings, making the identification of a practical pp-wave magnet a central pursuit in spintronics. The layered heavy-fermion oxypnictide CeNiAsO has been widely regarded as the prototypical platform to verify this paradigm, as its commensurate coplanar magnetic configuration is theoretically expected to induce a robust pp-wave band splitting. Here, we investigate the electronic structure of single-crystal CeNiAsO using ultra-low-temperature, high-resolution, and resonant angle-resolved photoemission spectroscopy (ARPES). Across the consecutive magnetic transitions into the ordered phases, our spectroscopic data reveal neither the expected band folding associated with a spin density wave nor any observable pp-wave band splitting, demonstrating that the conduction bands retain full Kramers degeneracy. By tracking the temperature dependence of the Ce 4ff spectral weight via resonant ARPES, we find no evidence of coherent c−fc-f hybridization near the Fermi level within the magnetically ordered states, confirming that the Ce 4ff electrons operate in the localized limit. Our findings establish a clear many-body constraint on projecting real-space magnetic symmetries onto momentum-space electronic bands, demonstrating that geometric symmetry classifications constitute a necessary framework but are not a sufficient condition for nonrelativistic spin splittings in the presence of strong electronic correlations.

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