Odd-Parity Magnons

Abstract: Magnons, as charge-neutral spin excitations, can transport spin information without Joule heating and therefore offer a promising platform for low-power spintronics. However, in collinear magnets, the effective time-reversal symmetry forbids odd-parity magnon band splitting. Here we propose odd-parity magnons and establish a general mechanism for realizing them in collinear antiferromagnets. We provide a complete spin-point-group classification of odd-parity magnon splitting in two-dimensional collinear antiferromagnets by identifying the leading splitting types and their symmetry-allowed basis functions. This classification serves as a practical guide for searching for odd-parity magnons. We show that breaking effective time-reversal symmetry, for example by circularly polarized light or loop currents, can induce highly tunable $p$- and $f$-wave magnon splitting. In bilayer systems, the dynamical modulation can drive a topological magnon phase transition, accompanied by chiral edge modes and an abrupt jump in the magnon thermal Hall conductivity. Material-specific first-principles calculations further demonstrate the feasibility of this mechanism in real van der Waals antiferromagnets. Our study identifies the odd-parity magnons as a new class of spin excitations and provides a theoretical foundation for odd-parity magnons and ultrafast optically controlled topological magnonic devices.