Observation of Altermagnetic Order Switching in Bulk MnTe by Polarized Neutron Diffraction

Abstract: Altermagnetic order, characterized by the Néel vector, breaks time-reversal symmetry (TRS) even in the nonrelativistic limit. Although spin-polarized and anomalous transport phenomena emerge with this order, they are mutually compensated by TRS-connected antiphase domains with opposite Néel vectors. Here we employ polarized neutron diffraction to directly probe the altermagnetic order in MnTe. Pronounced nuclear-magnetic interference terms were observed, providing direct evidence of a net Néel vector in the bulk crystal. Moreover, a weak ferromagnetic moment (WFM), originating from relativistic spin-orbit coupling, was found to be coupled with the altermagnetic order. Both the altermagnetic order and the WFM can be switched by milli-Tesla-scale magnetic field cooling.