Toward Neutrino and Dark Matter Detection with Ancient Minerals: TEM Study of Heavy-Ion Tracks in Olivine

Abstract: Solar, supernova, and atmospheric neutrinos, and possibly weakly interacting massive particle (WIMP) dark matter, have been interacting in the Earth beneath our feet for billions of years. The ''paleo-detector'' technique seeks to detect and characterize the induced crystalline defects from these events, in particular from energetic nuclear recoils, which in some minerals can be preserved on these timescales. Such defects can manifest as nuclear recoil tracks, on the order of a few nanometers wide and extending up to hundreds of microns in length, which can be detected with nanoscale-resolution microscopy. In order to test the feasibility of the paleo-detector technique and to study the formation and morphology of track defects in promising mineral candidates like olivine, we use ion irradiation to artificially implant tracks to effectively mimic astrophysical particle interactions. We present a study of heavy-ion track width as a function of depth, which we relate to ion energy, in an olivine crystal irradiated with 15 MeV Au$^{+5}$ using scanning transmission electron microscopy (STEM). Unlike previous studies, which measure tracks at the surface of the irradiated sample, we instead take measurements at various target depths via focused ion-beam sectioning of the irradiated sample. No etching techniques are used to enhance the tracks. In addition, we provide a comparison to predictions from simulations using SRIM software and previous results with a variety of ion species and energies. Notably, we find that a significant change in track continuity across the energy range studied (0.4-12.9 MeV) is indicative of the transition between electronic and nuclear stopping power dominance, consistent with the simulations' predictions. Overall, the tracks produced in olivine indicate that this mineral is an attractive candidate for paleo-detection, with robust track creation at the MeV scale.