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Microscopic origin of pp-wave magnetism

Published 10 Mar 2026 in cond-mat.mes-hall, cond-mat.mtrl-sci, and cond-mat.str-el | (2603.09736v1)

Abstract: PP-, ff-, or hh-wave antialtermagnets yield large non-relativistic spin splitting with out-of-plane spin polarization in momentum space perpendicular to the coplanar non-collinear local magnetic moments. We provide a microscopic explanation of this unconventional spin polarization by linking it to a previously overlooked site-compensated spin density that orders antiparallel when projected onto opposite momenta. We verify this result both by model derivation of the out-of-plane momentum-space spin polarization being proportional to the direct-space cross product of the coplanar non-collinear spin order, as well as by ab initio calculations in the material candidate CeNiAsO. By providing a general classification and analytic expression for the spin polarization of all spinful two-site tight-binding Hamiltonians, we reveal the momentum-resolved spin polarization as a probe of the Bloch-state geometry arising from spin-site coupling. Furthermore, our approach allows for geometric distinction between ferro-, alter-, and antialtermagnets. Our results provide a quantitative guidance for quantized out-of-plane momentum-space spin polarization and large spin splitting, and construction principles for antialtermagnets.

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