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Anisotropic Electronic Correlations in the Spin Density Wave State of La3_3Ni2_2O7_7

Published 8 Feb 2026 in cond-mat.supr-con | (2602.07998v1)

Abstract: The bilayer nickelate superconductor La<em>3<em>3Ni2_2O7_7 undergoes a density wave transition near 150 K that has attracted intensive scrutiny, yet its microscopic origin remains elusive. Here we report polarization-resolved electronic Raman scattering measurements on high-quality single crystals of La3_3Ni2_2O7_7. Below 150\,K, we observe a pronounced, symmetry-dependent redistribution of spectral weight in B</em>1g</em>{1g} and B2g_{2g} channels, consistent with the formation of spin-density-wave (SDW) gaps. Quantitative analysis reveals momentum-selective SDW gap amplitudes, with intermediate-to-strong coupling near X/Y points of the Brillouin zone and weaker coupling along the diagonal direction, indicating an unconventional SDW driven by anisotropic electronic correlations. Our results establish the electronic character of the SDW in La3_3Ni2_2O7_7, and provide a microscopic foundation for understanding the emergence of high-temperature superconductivity under pressure in nickelates.

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