Néel-Vector-Orientation Induced Intrinsic Half-Metallicity in Two-Dimensional Altermagnets

Abstract: Altermagnets combine zero net magnetization with giant spin splitting, enabling spin-polarized transport without strong spin-orbit coupling (SOC). Deterministically selecting the conducting spin channel, however, requires breaking the 90 degree rotation and time-reversal antisymmetry (C4zT). Using standard axial vector transformation rules as preliminaries, we show that in monolayer Ta2TeSeO this can be achieved naturally and tuned in a symmetry efficient way by rotating the Neel vector. Without considering the Neel vector, Ta2TeSeO has one pair of mirror protected spin polarized Weyl points in each spin channel. Aligning the Neel vector along the crystallographic x or y direction breaks the mirror symmetry Mx or My, inducing selective mirror symmetry breaking that keeps one spin sector gapless and opens a gap in the opposite spin, yielding fully spin polarized transport. The C2z symmetry breaking makes the preserved two Weyl points inequivalent, turning the half semimetal into a half metallic state. The same orientation selective symmetry reduction applies to lattice vibrations, implying phonon chirality splitting. Owing to the near degenerate in plane anisotropy, reversible zero moment switching is achievable with minute in plane strain or weak magnetic fields, and the lattice coupling suggests control by circularly polarized light. The mechanism extends to other two dimensional decorated Lieb altermagnets lacking horizontal mirror Mz, providing a general low power route to spin filtering and logic.