Investigating Solid-Fluid Phase Coexistence in DC Plasma Bilayer Crystals: The Role of Particle Pairing and Mode Coupling

Abstract: This article presents a detailed investigation of solid-fluid phase coexistence in a bilayer dusty plasma crystal subjected to varying confinement ring bias voltages in a DC glow discharge argon plasma. Melamine formaldehyde particles were employed to form a stable, hexagonally ordered bilayer crystal within a confinement ring electrically isolated from the grounded cathode. By systematically adjusting the confinement ring bias, a distinct phase coexistence emerged: it is characterized by a fluid-like melted core surrounded by a solid crystalline periphery. Crucially, analysis of the phonon spectra revealed frequency shifts that deviate significantly from the predictions of classical monolayer Mode-Coupling Instability (MCI) theory. Stability analysis further demonstrated that dynamic interlayer particle pairing and non-reciprocal interactions play a pivotal role in destabilizing the bilayer structure. These findings highlight previously underappreciated mechanisms driving the melting transition in bilayer dusty plasmas, offering a more comprehensive understanding of phase behavior in complex plasma systems. The results underscore the importance of interlayer coupling and confinement effects in tuning structural transitions.