Observation of surface superconductivity in bulk polycrystalline MoS2 induced by electric double-layer doping

Abstract: We report the observation of electric-field-induced superconductivity on the surface of bulk polycrystalline MoS2 using electric double-layer doping. A gate voltage applied in an ionic liquid environment systematically increased carrier density, leading to an insulator-to-metal transition and a sharp resistance drop at low temperatures, indicating superconductivity. The onset temperature of superconductivity strongly depended on carrier density inferred from conductance, showing a significant increase and eventual saturation. Unlike prior studies limited to single-crystalline MoS2, our results demonstrate that superconductivity can also be electrostatically induced in polycrystalline systems, broadening the scope for exploring gate-controlled superconductivity in a wider range of materials.