Can We Conjugate the Orbital Angular Momentum of a Single Photon with Nonlinear Optics? A Theoretical Analysis

Abstract: Stimulated parametric down-conversion (StimPDC) produces an idler beam that exhibits a phase conjugate of the spatial structure of the classical seed beam. Extending this effect to the single-photon regime can, in principle, enable the control of the orbital angular momentum of single photons. However, its experimental implementation remains challenging due to the lower photon flux of realistic single-photon sources compared to a classical pump beam, which causes the StimPDC process to occur less frequently compared to its spontaneous counterpart. To overcome this, we propose a cascaded parametric down-conversion scheme, in which the signal photon from a spontaneously down-converted pair seeds the StimPDC process, while the idler photon heralds the seed's presence. This configuration uses coincidence detection to effectively post-select for stimulated events among the background of spontaneous contributions. We show that phase conjugation at the single-photon level manifests as a bias towards equal orbital angular momentum between the heralding idler and the stimulated idler. Our results offer a practical route to manipulate single-photon correlations in the orbital angular momentum degree of freedom and could have implications for applications such as free-space quantum communication and quantum-enhanced sensing.