On the Néel Vector Dependence of X-ray Magnetic Circular Dichroism in Altermagnets

Abstract: Dependence of x-ray magnetic circular dichroism on the experimental geometry is described by a frequency-dependent Hall vector. Using group theory, we derive a general relationship between the Hall vector and the orientation of the N\'eel vector $\bL$ in altermagnets within the free valence spin (FVS) approximation, where the spin-orbit coupling of the valence electrons and their exchange interaction with the core electrons are neglected. For a given spin point group, the full $\bL$-dependence of the Hall vector can be expressed in terms of several irreducible spectral functions. This derivation generalizes earlier results for the special cases of MnTe and MnF$_2$. Depending on the system symmetry, XMCD in the FVS approximation may be present, emerge only when the neglected terms are included, or be completely forbidden.