Spin Correlations in Recirculating Multipass Alkali Cells for Advancing Quantum Magnetometry

Abstract: Multipass cells are critical components in a variety of quantum technologies, including atomic magnetometers and optical quantum memories, due to their ability to achieve long optical paths within compact volumes. In optical magnetometry, increasing the optical depth through multipass geometries enhances sensitivity by reducing photon shot noise and enabling quantum nondemolition (QND) detection. In this work, we present a novel recirculating multipass alkali cell that improves the active-to-cell volume ratio and minimizes beam spot overlap, thereby addressing spin noise limitations inherent in conventional cylindrical Herriott cavity designs. We develop and validate an analytical model based on the ABCD matrix method to predict beam spot positions, sizes, and astigmatism effects, with results confirmed through Zemax simulations. In addition, we introduce a general analytical model for analyzing spin correlation noise in multipass alkali cells, incorporating both astigmatism and spatial intensity distribution-features not addressed in existing models. By deriving the spin noise time-correlation function and spectrum, we reveal how power intensity profiles contribute to spin diffusion noise. Our analysis demonstrates that the recirculating cell offers improved beam coverage, reduced spot overlap, and enhanced spin correlation-particularly when using concave mirrors with longer focal lengths. Furthermore, we show that avoiding tightly focused, high-intensity regions can significantly suppress spin diffusion noise. These findings establish the recirculating cell design as a practical and high-performance solution for advancing the precision of atomic sensors and other multipass cavity-based quantum devices.