Novel entangled dimer state in the Shastry-Sutherland magnet Yb$_2$Be$_2$SiO$_7$

Abstract: The Shastry-Sutherland lattice (SSL) magnet, with antiferromagnetic intradimer and interdimer Heisenberg exchange, is known to host an antisymmetric singlet ground state when the intradimer exchange is dominant. Rare-earth-based SSL systems with strong spin-orbit coupling offer the opportunity for tuning their magnetic properties by using magnetic anisotropy as a control knob. Here, we present bulk characterization and neutron scattering measurements of the SSL material Yb$_2$Be$_2$SiO$_7$. We find that the Yb$^{3+}$ ions can be described by an effective spin-1/2 model at low temperatures and the system does not show signs of magnetic order down to 50 mK. The magnetization, heat capacity, and neutron spectroscopy data can be well-described by an isolated dimer model with highly anisotropic exchange that stabilizes a singlet ground state with the symmetric wavefunction up/up - down/down. Our results show that strong spin-orbit coupling can induce novel entangled states of matter on the SSL.