Quantitative imaging of nonlinear spin-wave propagation using diamond quantum sensors

Abstract: Spin waves propagating in magnetic materials exhibit nonlinear behavior due to the competition between excitation and relaxation at large amplitudes, providing an attractive platform for exploring nonlinear wave dynamics. In particular, spin waves with a non-zero wavenumber that carry momentum undergo nonlinear relaxation and experience wavenumber modulation in the nonlinear regime. We image the nonlinear spin-wave propagation in two yttrium iron garnet thin films with distinct spin-wave decay rates using a wide-field quantum diamond microscope. We obtain quantitative distributions of spin-wave amplitude and phase in varying excitation microwave strength. As a result, we observe a threshold in the spin-wave amplitude beyond which nonlinear effects become evident and confirm that this threshold is consistent with theoretical predictions based on four-magnon scattering for both samples. Moreover, as the amplitude of the spin waves increases, modulation of the wavenumber is observed across the field of view. We attribute this modulation primarily to the spin waves generated by multi-magnon scattering. Our quantitative measurements provide a pathway for visualizing nonlinear spin-wave dynamics and are crucial for deepening our understanding of the underlying mechanisms.