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Possible quantum spin liquid state of CeTa$_7$O$_{19}$

Published 2 Mar 2025 in cond-mat.str-el and cond-mat.mtrl-sci | (2503.00752v2)

Abstract: CeTa$7$O${19}$ is a recently found two-dimensional triangular lattice antiferromagnet without showing magnetic order. We grew high-quality CeTa$7$O${19}$ single crystals and studied the low-temperature magnetic susceptibility, specific heat and thermal conductivity. The dc magnetic susceptibility and magnetization reveal its nature of effective spin-1/2, easy axis anisotropy, and antiferromagnetic spin coupling. The ultralow-temperature ac susceptibility and specific heat data indicate the absence of any phase transition down to 20 mK. The ultralow-temperature thermal conductivity ($\kappa$) at zero magnetic field exhibits a non-zero residual term $\kappa_0/T =$ 0.0056 W/K$2$m. Although the magnetic field dependence of $\kappa$ is rather weak, the 14 T thermal conductivity shows an essential zero residual term. All these results point to a possible ground state of quantum spin liquid.

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