Solid and hollow plasmonic nanoresonators for carrier envelope phase read-out (2404.11940v1)

Abstract: The geometry of various plasmonic nanoantennae was numerically optimized to maximize their sensitivity to the carrier envelope phase (CEP) of the exciting ultra-short laser pulses. To verify the CEP sensitivity, the near-field response of the investigated nanoantennae was analyzed by combining frequency and time-domain numerical computations. The simulation methodology, capable of accurately calculating the time-dependent photocurrent stem from optical field emission, enabled the determination and optimization of all key parameters characterizing and governing the CEP dependence of the near-field responses. Three-types of structures were inspected, including individual triangular and teardrop-shaped nanoantennae and plasmonic lenses consisting of three hemispheres with gradually decreasing diameters. All structure types were optimized in solid and hollow compositions of gold nanoresonators as well. It was shown that hollow /solid singlets produce the largest /intermediate CEP dependent - to - CEP independent integrated current components' ratio, while their absolute CEP dependent integrated currents were the smallest /intermediate among the optimized structures. The highest /intermediate CEP sensitivity was achieved via solid plasmonic lenses due to their very large absolute CEP dependent integrated photocurrent originating from huge near-field enhancement in the nanogaps, while the integrated current components' ratio was smaller than for counterpart singlets.