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Phase Coexistence and Transitions between Antiferromagnetic and Ferromagnetic States in a Synthetic Antiferromagnet (2401.16273v2)

Published 29 Jan 2024 in cond-mat.mes-hall

Abstract: In synthetic antiferromagnets (SAFs) the combination of antiferromagnetic order and synthesis using conventional sputtering techniques is combined to produce systems that are advantageous for spintronics applications. Here we present the preparation and study of SAF multilayers possessing both perpendicular magnetic anisotropy and the Dzyaloshinskii-Moriya interaction. The multilayers have an antiferromagnetically (AF) aligned ground state but can be forced into a full ferromagnetic (FM) alignment by applying an out-of-plane field $\sim 100$~mT. We study the spin textures in these multilayers in their ground state as well as around the transition point between the AF and FM states, at fields $\sim 40$~mT, by imaging the spin textures using complementary methods: photo-emission electron, magnetic force, and Lorentz transmission electron microscopies. The transformation into a FM state by field proceeds by a nucleation and growth process, where first skyrmionic nuclei form, which broaden into regions containing a FM-aligned labyrinth pattern that eventually occupies the whole film. This process remarkably occurs without any significant change in the net magnetic moment of the multilayer. The mix of AF- and FM-aligned regions on the micron scale in the middle of this transition is reminiscent of a first-order phase transition that exhibits phase coexistence. These results are important for guiding the design of spintronic devices using chiral magnetic textures made from SAFs.

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