Metadynamics calculations of the effect of thermal spin fluctuations on skyrmion stability
Abstract: The stability of magnetic skyrmions has been investigated in the past, but mostly in the absence of thermal fluctuations. However, thermal spin fluctuations modify the magnetic properties (exchange stiffness, Dzyaloshinskii-Moriya interaction (DMI) and anisotropy) that define skyrmion stability. Thermal magnons also excite internal skrymion dynamics, deforming the skyrmion shape. Entropy has also been shown to modify skyrmion lifetimes in experiments, but is absent or approximated in previous studies. Here we use metadynamics to calculate the free energy surface of a magnetic thin film in terms of the topological charge and magnetization. We identify the free energy minima corresponding to different spin textures and the lowest energy paths between the ferromagnetic and single skyrmion states. We show that at low temperatures the lowest free energy barrier is a skyrmion collapse process. However, this energy barrier increases with temperature. An alternative path, where a singularity forms on the skrymion edge, has a larger free energy barrier at low temperatures but decreases with increasing temperature and eventually becomes the lowest energy barrier.
- A. Fert, N. Reyren, and V. Cros, Magnetic skyrmions: advances in physics and potential applications, Nat. Rev. Mater. 2, 17031 (2017).
- A. N. Bogdanov and C. Panagopoulos, Physical foundations and basic properties of magnetic skyrmions, Nat. Rev. Phys. 2, 492 (2020).
- N. Nagaosa and Y. Tokura, Topological properties and dynamics of magnetic skyrmions, Nat. Nanotechnol. 8, 899 (2013).
- H. Y. Yuan and X. R. Wang, Skyrmion Creation and Manipulation by Nano-Second Current Pulses, Sci. Rep. 6, 22638 (2016).
- J. Iwasaki, M. Mochizuki, and N. Nagaosa, Current-induced skyrmion dynamics in constricted geometries, Nat. Nanotechnol. 8, 742 (2013).
- O. Petrova and O. Tchernyshyov, Spin waves in a skyrmion crystal, Phys. Rev. B 84, 214433 (2011).
- M. Mochizuki, Spin-Wave Modes and Their Intense Excitation Effects in Skyrmion Crystals, Phys. Rev. Lett. 108, 017601 (2012).
- S.-Z. Lin, C. D. Batista, and A. Saxena, Internal modes of a skyrmion in the ferromagnetic state of chiral magnets, Phys. Rev. B 89, 024415 (2014).
- A. Laio and M. Parrinello, Escaping free-energy minima, Proc. Natl. Acad. Sci. 99, 12562 (2002).
- A. Barducci, M. Bonomi, and M. Parrinello, Metadynamics, WIREs Comput. Mol. Sci. 1, 826 (2011).
- B. Nagyfalusi, L. Udvardi, and L. Szunyogh, First principles and metadynamics study of the spin-reorientation transition in Fe/Au(001) films, J. Phys.: Conf. Ser. 903, 012016 (2017).
- B. Nagyfalusi, L. Udvardi, and L. Szunyogh, Metadynamics study of the temperature dependence of magnetic anisotropy and spin-reorientation transitions in ultrathin films, Phys. Rev. B 100, 174429 (2019).
- J. Tóbik, R. Martoňák, and V. Cambel, Free-energy landscapes in magnetic systems from metadynamics, Phys. Rev. B 96, 140413 (2017).
- D. P. Landau and K. Binder, A guide to Monte Carlo simulations in statistical physics (Cambridge University Press, 2021).
- A. Laio and F. L. Gervasio, Metadynamics: a method to simulate rare events and reconstruct the free energy in biophysics, chemistry and material science, Rep. Prog. Phys. 71, 126601 (2008).
- J.-V. Kim and J. Mulkers, On quantifying the topological charge in micromagnetics using a lattice-based approach, IOP SciNotes 1, 025211 (2020).
- Using the ‘geometrical definition’ of topological charge as a summation over plaquettes [36] always produces an integer and therefore cannot be used as a CV for metadynamics.
- A. Laio, G. Martinelli, and F. Sanfilippo, Metadynamics surfing on topology barriers: the CPN−1𝐶superscript𝑃𝑁1CP^{N-1}italic_C italic_P start_POSTSUPERSCRIPT italic_N - 1 end_POSTSUPERSCRIPT case, J. High Energy Phys. 2016, 89.
- C. Bonanno, C. Bonati, and M. D’Elia, Topological properties of CPN−1𝐶superscript𝑃𝑁1CP^{N-1}italic_C italic_P start_POSTSUPERSCRIPT italic_N - 1 end_POSTSUPERSCRIPT models in the large-N𝑁Nitalic_N limit, J. High Energy Phys. 2019, 3.
- G. Bussi and A. Laio, Using metadynamics to explore complex free-energy landscapes, Nat. Rev. Phys. 2, 200 (2020).
- A. Barducci, G. Bussi, and M. Parrinello, Well-Tempered Metadynamics: A Smoothly Converging and Tunable Free-Energy Method, Phys. Rev. Lett. 100, 020603 (2008).
- I. Marcos-Alcalde, E. López-Viñas, and P. Gómez-Puertas, MEPSAnd: minimum energy path surface analysis over n-dimensional surfaces, Bioinformatics 36, 956 (2020).
- I. Marcos-Alcalde, E. López-Viñas, and P. Gómez-Puertas, MEPSAnd v1.6 (2022).
- L. Rózsa, U. Atxitia, and U. Nowak, Temperature scaling of the Dzyaloshinsky-Moriya interaction in the spin wave spectrum, Phys. Rev. B 96, 094436 (2017).
- B. Berg and M. Lüscher, Definition and statistical distributions of a topological number in the lattice O(3) σ𝜎\sigmaitalic_σ-model, Nucl. Phys. B 190, 412 (1981).
Paper Prompts
Sign up for free to create and run prompts on this paper using GPT-5.
Top Community Prompts
Collections
Sign up for free to add this paper to one or more collections.