Interplay between multi-spin and chiral spin interactions on triangular lattice (2306.03478v1)

Abstract: We investigate the spin-$\frac{1}{2}$ nearest-neighber Heisenberg model with the four-site ring-exchange $J_4$ and chiral interaction $J_\chi$ on the triangular lattice by using the variational Monte Carlo method. The $J_4$ term induces the quadratic band touching (QBT) quantum spin liquid (QSL) with only a $d+id$ spinon pairing (without hopping term), the nodal $d$-wave QSL and U(1) QSL with a finite spinon Fermi surface progressively. The effect of the chiral interaction $J_\chi$ can enrich the phase diagram with two interesting chiral QSLs (topological orders) with the same quantized Chern number $\mathcal{C} = \frac{1}{2}$ and ground-state degeneracy GSD = 2, namely the U(1) chiral spin liquid (CSL) and Z$2$ $d+id$-wave QSL. The nodal $d$-wave QSL is fragile and will turn to the Z$_2$ $d+id$ QSL with any finite $J\chi$ within our numerical calculation. However, in the process from QBT to the Z$2$ $d+id$ QSL with the increase of $J\chi$, an exotic crossover region is found. In this region, the previous QBT state acquires a small hopping term so that it opens a small gap at the otherwise band touching points, and leads to an energy minimum which is energetically more favorable compared to another competitive local minimum from the Z$2$ $d+id$ QSL. We dub this state as the proximate QBT QSL and it gives way to the Z$_2$ $d+id$ QSL eventually. Therefore, the cooperation of the $J_4$ and $J\chi$ terms favors mostly the Z$_2$ $d+id$-wave QSL, so that this phase occupies the largest region in the phase diagram.