Interplay of magnetic field and magnetic impurities in Ising superconductors
Abstract: Phonon-driven -wave superconductivity is fundamentally antagonistic to uniform magnetism, and field-induced suppression of the critical temperature is one of its canonical signatures. Examples of the opposite are unique and require fortuitous cancellations and very fine parameter tuning. The recently discovered Ising superconductors violate this rule: an external magnetic field applied in a certain direction does not suppress superconductivity in an ideal, impurity-free material. We propose a simple and experimentally accessible system where the effects of spin-conserving and spin-flip scattering can be studied in a controlled way, namely NbSe monolayers dosed with magnetic $3d$ atoms. We predict that the critical temperature is slightly increased by an in-plane magnetic field in NbSe dosed with Cr. Due to the band spin splitting, magnetic spin-flip scattering requires a finite momentum transfer, while spin-conserving scattering does not. If the magnetic anisotropy is easy-axis, an in-plane field reorients the impurity spins and transforms spin-conserving scattering into spin-flip. The critical temperature is enhanced if the induced magnetization of NbSe has a substantial long-range component, as is the case for Cr ions.
- I. I. Mazin and the PRX editors, Editorial: Altermagnetism—a new punch line of fundamental magnetism, Phys. Rev. X 12, 040002 (2022), see a more complete version at https://arxiv.org/abs/2212.13110.
- L. Šmejkal, J. Sinova, and T. Jungwirth, Beyond conventional ferromagnetism and antiferromagnetism: A phase with nonrelativistic spin and crystal rotation symmetry, Phys. Rev. X 12, 031042 (2022).
- D. Wickramaratne and I. I. Mazin, Effect of alloying in monolayer niobium dichalcogenide superconductors, Nat. Commun. 13, 2376 (2022).
- A. A. Abrikosov and L. P. Gor’kov, Contribution to the theory of superconducting alloys with paramagnetic impurities, Zh. Eksp. Teor. Fiz. 39, 1781 (1960).
- V. Jaccarino and M. Peter, Ultra-high-field superconductivity, Phys. Rev. Lett. 9, 290 (1962).
- S. Ilić, J. S. Meyer, and M. Houzet, Enhancement of the upper critical field in disordered transition metal dichalcogenide monolayers, Phys. Rev. Lett. 119, 117001 (2017).
- D. Möckli, M. Haim, and M. Khodas, Magnetic impurities in thin films and 2d ising superconductors, Journal of Applied Physics 128, 053903 (2020).
- J. J. Hauser, M. Robbins, and F. J. DiSalvo, Effect of 3d3𝑑3d3 italic_d impurities on the superconducting transition temperature of the layered compound NbSe2, Phys. Rev. B 8, 1038 (1973).
- L. Bulaevskii, A. Guseinov, and A. Rusinov, Superconductivity in crystals without symmetry centers, Zh. Eksp. Teor. Fiz. 71, 2356 (1976).
- D. Shaffer, F. J. Burnell, and R. M. Fernandes, Weak-coupling theory of pair density wave instabilities in transition metal dichalcogenides, Phys. Rev. B 107, 224516 (2023).
- E. Sosenko, J. Zhang, and V. Aji, Unconventional superconductivity and anomalous response in hole-doped transition metal dichalcogenides, Phys. Rev. B 95, 144508 (2017).
- M. Haim, A. Levchenko, and M. Khodas, Mechanisms of in-plane magnetic anisotropy in superconducting nbse2subscriptnbse2{\mathrm{nbse}}_{2}roman_nbse start_POSTSUBSCRIPT 2 end_POSTSUBSCRIPT, Phys. Rev. B 105, 024515 (2022).
- D. Möckli and M. Khodas, Robust parity-mixed superconductivity in disordered monolayer transition metal dichalcogenides, Phys. Rev. B 98, 144518 (2018).
- M. Tinkham, Introduction to Superconductivity, 2nd ed. (Dover Publications, 2004).
- A. A. Golubov and I. I. Mazin, Effect of magnetic and nonmagnetic impurities on highly anisotropic superconductivity, Phys. Rev. B 55, 15146 (1997).
- P. E. Blöchl, Projector augmented-wave method, Phys. Rev. B 50, 17953 (1994).
- G. Kresse and J. Hafner, Ab initio molecular dynamics for liquid metals, Phys. Rev. B 47, 558 (1993).
- G. Kresse and J. Furthmüller, Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set, Phys. Rev. B 54, 11169 (1996).
- J. P. Perdew, K. Burke, and M. Ernzerhof, Generalized gradient approximation made simple, Phys. Rev. Lett. 77, 3865 (1996).
- T. Ozaki, Variationally optimized atomic orbitals for large-scale electronic structures, Phys. Rev. B 67, 155108 (2003).
- Openmx 3.9, http://www.openmx-square.org.
- A. I. Liechtenstein, V. I. Anisimov, and J. Zaanen, Density-functional theory and strong interactions: Orbital ordering in mott-hubbard insulators, Phys. Rev. B 52, R5467 (1995).
- S. Das and I. I. Mazin, Quantitative assessment of the role of spin fluctuations in 2D ising superconductor NbSe2, Computational Materials Science 200, 110758 (2021).
Paper Prompts
Sign up for free to create and run prompts on this paper.