Charge dynamics in spintronic THz emitters (2208.07616v1)

Abstract: We show that to correctly describe the ultrafast currents in spintronic THz emitters it is necessary to take charge equilibration into account. The charge current which is locally induced by a fs laser pulse and the inverse spin-Hall effect (ISHE) leads to ultrafast charging phenomena at the edge of the illuminated area. Subsequent discharging leads to a current backflow with a delay and a time constant that mainly depends on the conductivity of the emitter. On the one hand, only this delayed charge equilibration allows the detection of the primary current pulse via THz emission because an instantaneous backflow would cancel any far field emission. On the other hand, especially for longer light pulses the backflow can significantly change the emitted spectrum compared to the initial spin-current pulse by suppressing low frequency components. For the analysis of spin physics based on the charge current profile it is important to understand that the timing of the spin current cannot be inferred from the charge current unless the contribution by the ISHE and the backflow can be deconvoluted.