Spin waves and magnetic exchange Hamiltonian in CrSBr

Abstract: CrSBr is an air-stable 2D van der Waals semiconducting magnet with great technological promise, but its atomic-scale magnetic interactions -- crucial information for high-frequency switching -- are poorly understood. We present an experimental study to determine the CrSBr magnetic exchange Hamiltonian and bulk magnon spectrum. We confirm the $A$-type antiferromagnetic order using single crystal neutron diffraction. We also measure the magnon dispersions using inelastic neutron scattering and rigorously fit the excitation modes to a spin wave model. The magnon spectrum is well described by an intra-plane ferromagnetic Heisenberg exchange model with seven nearest in-plane exchanges. This fitted exchange Hamiltonian enables theoretical predictions of CrSBr behavior: as one example, we use the fitted Hamiltonian to predict the presence of chiral magnon edge modes with a spin-orbit enhanced CrSBr heterostructure.