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Magnetic properties of the itinerant ferromagnet LaCrGe3 under pressure studied by 139La NMR

Published 7 May 2021 in cond-mat.str-el | (2105.03479v1)

Abstract: <sup>139<sup>{139}La nuclear magnetic resonance (NMR) measurements under pressure (p=0−2.64p = 0-2.64 GPa) have been carried out to investigate the static and dynamic magnetic properties of the itinerant ferromagnet LaCrGe<em>3<em>3. <sup>139<sup>{139}La-NMR spectra for all measured pressures in the ferromagnetically ordered state show a large shift due to the internal field induction ∣|B{\rm int}∣| ∼\sim 4 T at the La site produced by Cr ordered moments. The change in BintB_{\rm int} by less than 5\% with pp up to 2.64~GPa indicates that the Cr 3dd moments are robust under pressure. The temperature dependence of NMR shift and BintB_{\rm int} suggest that the ferromagnetic order develops below ∼\sim 50~K under higher pressures in a magnetic field of ∼\sim 7.2 T. Based on the analysis of NMR data using the self-consistent-renormalization (SCR) theory, the spin fluctuations in the paramagnetic state well above TCT_{\rm C} are revealed to be three dimensional ferromagnetic throughout the measured pp region.

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