Vectorial polaritons in the quantum motion of a levitated nanosphere

Abstract: The strong coupling between elementary excitations of the electromagnetic field (photons) and quantized mechanical vibrations (phonons) produces hybrid quasi-particle states, known as phonon-polaritons. Their typical signature is the avoided crossing between the eigenfrequencies of the coupled system, as paradigmatically illustrated by the Jaynes-Cummings Hamiltonian, and observed in quantum electrodynamics experiments where cavity photons are coupled to atoms, ions, excitons, spin ensambles and superconducting qubits. In this work, we demonstrate the generation of phonon-polaritons in the quantum motion of an optically-levitated nanosphere. The particle is trapped in high vacuum by an optical tweezer and strongly coupled to a single cavity mode by coherent scattering of the tweezer photons. The two-dimensional motion splits into two nearly-degenerate components that, together with the optical cavity mode, define an optomechanical system with three degrees-of-freedom. As such, when entering the strong coupling regime, we observe hybrid light-mechanical states with a dispersion law typical of tripartite quantum systems. Remarkably, the independent components of motion here identify a physical vibration direction on a plane that, similarly to the polarization of light, confers a vectorial nature to the polariton field. Our results pave the way to novel protocols for quantum information transfer between photonic and phononic components and represent a key-step towards the demonstration of optomechanical entangled states at room temperature.