Intermittent dilation and its coupling to stress in discontinuous shear thickening suspensions

Abstract: We investigate dilation-induced surface deformations in a Discontinuous Shear Thickening (DST) suspension to determine the relationship between dilation and stresses in DST. Video is taken at two observation points on the surface of the suspension in a rheometer while shear and normal stresses are measured. A roughened surface of the suspension is observed as particles poke through the liquid-air interface, corresponding to dilation. Dilation events are found to be intermittent and localized spatially. Shear and normal stresses also fluctuate between high- and low-stress states, and dilation is observed frequently in the high stress state. On the other hand, a complete lack of dilation is observed when the stresses remain at low values for a several seconds. Dilation is most prominent while the stresses grow from the low-stress state to the high-stress state, and the dilated region tends to span the entire surface by the end of the stress growth period. Dilation is found only at stresses and shear rates in and above the shear thickening range. These observed relations between surface dilation and stresses confirm that dilation and stresses are coupled in the high-stress state of DST.