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Magnetic structure of the antiferromagnetic Kondo lattice compounds CeRhAl4Si2 and CeIrAl4Si2

Published 23 Mar 2015 in cond-mat.str-el | (1503.06860v1)

Abstract: We have investigated the magnetic ground state of the antiferromagnetic Kondo-lattice compounds CeMAl${4}$Si${2}$ (M = Rh, Ir) using neutron powder diffraction. Although both of these compounds show two magnetic transitions $T_{N1}$ and $T_{N2}$ in the bulk properties measurements, evidence for magnetic long-range order was only found below the lower transition $T_{N2}$. Analysis of the diffraction profiles reveals a commensurate antiferromagnetic structure with a propagation vector $\mathbf{k}$= (0, 0, 1/2). The magnetic moment in the ordered state of CeRhAl${4}$Si${2}$ and CeIrAl${4}$Si${2}$ were determined to be 1.14(2) and 1.41(3) $\mu_{B}$/Ce, respectively, and are parallel to the crystallographic $c$-axis in agreement with magnetic susceptibility measurements.

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