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Attosecond streaking of Cohen-Fano interferences in the photoionization of H$_2^+$

Published 24 Jan 2014 in physics.atom-ph, physics.atm-clus, and physics.chem-ph | (1401.6233v1)

Abstract: We present the first numerical simulation of the time delay in the photoionization of the simplest diatomic molecule H$_2+$ as observed by attosecond streaking. We show that the strong variation of the Eisenbud-Wigner-Smith time delay as a function of energy and emission angle becomes observable in the streaking time shift provided laser field-induced components are accounted for. The strongly enhanced photoemission time shifts are traced to destructive Cohen-Fano (or two-center) interferences. Signatures of these interferences in the streaking trace are shown to be enhanced when the ionic fragments are detected in coincidence.

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