Microdroplet oscillations during optical pulling

Abstract: It was recently shown theoretically that it is possible to pull a spherical dielectric body towards the source of a laser beam [Nature Photonics {\bf 5}, 531 (2011)], a result with immediate consequences to optical manipulation of small droplets. Optical pulling can be realised e.g.\ using a diffraction free Bessel beam, and is expected to be of great importance in manipulation of microscopic droplets in micro- and nanofluidics. Compared to conventional optical pushing, however, the radio of optical net force to stress acting on a droplet is much smaller, increasing the importance of oscillations. We describe the time-dependent surface deformations of a water microdroplet under optical pulling to linear order in the deformation. Shape oscillations have a lifetime in the order of microseconds for droplet radii of a few micrometers. The force density acting on the initially spherical droplet is strongly peaked near the poles on the beam axis, causing the deformations to take the form of jet-like protrusions.