Magneto-electric effect in NdCrTiO5

Abstract: We have measured the dielectric constant and the pyroelectric current of orthorhombic (space group $Pbam$) NdCrTiO$5$ polycrystalline samples. The dielectric constant and the pyroelectric current show features associated with ferroelectric transitions at the antiferromagnetic transition temperature ($T{\text{N}}$ = 21 K). The effect of magnetic fields is to enhance the features almost linearly up to the maximum measured field (7 T) with a spontaneous polarization value of $\sim 3.5 \mu$C/m$^2$. Two possible scenarios, the linear magnetoelectric effect and multiferroicity (antiferromagnetism + ferroelectricity), are discussed as possible explanations for the observations.