Modelling of optical traps for aerosols

Abstract: Experimental observations suggest that there are differences between the behavior of particles optically trapped in air and trapped in a liquid phase. We present a modified version of Mie Debye Spherical Aberration theory to numerically simulate such optical system in attempt to explain and predict these effects. The model incorporates Mie scattering and focussing of the trapping beam through media of stratified refractive index. Our results show a geometrical optics approach cannot correctly describe our system and that spherical aberration must be included. We successfully qualitatively explain the observed phenomena and those of other authors, before discussing the limits of our experimental techniques and methods to improve it. We draw the important conclusion that when optically trapping aerosols the system does not behave as a true `optical tweezers', varying between levitation and single beam gradient force trapping depending on particle and beam parameters.