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Bulk magnetic order in a two dimensional Ni1+/Ni2+ (d9/d8) nickelate, isoelectronic with superconducting cuprates

Published 16 Mar 2010 in cond-mat.str-el and cond-mat.supr-con | (1003.3276v1)

Abstract: Bulk magnetic order in two dimensional La4Ni3O8 nickelate with Ni1+/Ni2+ (d9/d8), isoelectronic with superconducting cuprates is demonstrated experimentally and theoretically. Magnetization, specific heat and 139La NMR evidence a transition at 105 K to an antiferromagnetic state. Theoretical calculations by DFT relate the transition to a nesting instability of the Fermi surface with ordering wave-vector Q = [1/3, 1/3, 0].

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