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Waveguiding and Plasmon Resonances in Two-Dimensional Photonic Lattices of Gold and Silver Nanowires (0711.4553v1)

Published 28 Nov 2007 in physics.optics

Abstract: We report the fabrication of triangular lattices of parallel gold and silver nanowires of high optical quality, with diameters down to 500 nm and length-to-diameter ratios as high as 100,000. The nanowires are supported by a silica glass matrix and are disposed around a central solid glass core, i.e., a missing nanowire. These cm-long structures make it possible to trap light within an array of nanowires and characterize the plasmon resonances that form at specific optical frequencies. Such nanowire arrays have many potential applications, e.g., to imaging on the sub-wavelength scale.

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Summary

  • The paper demonstrates a novel waveguiding structure created by triangular arrays of gold and silver nanowires embedded in photonic crystal fibers.
  • The study employs multipole expansion to precisely map plasmon resonance wavelengths, revealing significant transmission dips at 940 nm for gold and 920 nm for silver.
  • The findings highlight distinct material-specific loss characteristics, paving the way for advanced sensor designs and miniaturized photonic devices.

An Analysis of Waveguiding and Plasmon Resonances in Two-Dimensional Photonic Lattices of Gold and Silver Nanowires

The paper, authored by Schmidt et al., focuses on the intricate fabrication and optical characterization of two-dimensional photonic lattices composed of gold and silver nanowires. These nanowires possess diameters as small as 500 nm and achieve length-to-diameter ratios as high as 100,000. Embedded in a silica glass matrix, these nanowires are arranged in a triangular lattice with a central solid glass core, acting as a missing nanowire. Such structuring facilitates light trapping and investigation of plasmon resonances at specific optical frequencies.

The discussed work is anchored in the fundamental physics of surface-plasmon-polaritons (SPPs), which occur at metal-dielectric interfaces due to substantial photon-electron interactions. These interactions foster significant field enhancements that could have far-reaching applications, particularly in enhancing the sensitivity of optical sensors and amplifying nonlinear effects.

One of the critical contributions of this paper is the demonstration of a novel waveguiding structure that comprises a triangular array of parallel metallic nanowires surrounding a central missing nanowire. This configuration serves the dual purpose of functioning as a waveguide and providing a means to probe the plasmonic properties of the nanowire array. This was realized through an innovative process where molten gold and silver were introduced into the narrow hollow channels of silica-based photonic crystal fibers (PCFs). The structures were then subjected to rigorous evaluation to understand their impact on waveguiding and resonance properties.

The paper provides quantitative metrics for the propagation of light within these nanowire arrays and characterizes spectral locations of surface-plasmon resonances (SPRs). Specifically, the research elucidates the dispersion and loss characteristics of the fundamental core-mode across different metal types and wire dimensions, employing a multipole expansion analysis to predict SPR wavelengths with high accuracy. Several significant experimental results were highlighted, including the finding that the transmission dips correlate strongly with nanowire thickness and arrangement.

Nanowire impedance to light at various thicknesses was found to vary significantly, with notable torques between the loss characteristics of gold and silver. For example, the studies revealed a major transmission dip at 940 nm for gold and 920 nm for silver. Besides, comparative analysis underscored a substantial variation in intrinsic losses between the two metals, accompanied by differing spectral characteristics due to unique complex dielectric constants.

The implications of this research are profound concerning the practical engineering of sub-wavelength imaging systems and potentially in the miniaturization of photonic components through very-large-scale integration (VLSI). The paper suggests the potential for application-driven design of nanowire arrays, exhibiting adaptability in sub-wavelength optical systems thanks to the choice of material and geometrical configurations.

In conclusion, the paper constitutes a substantial advancement in understanding the optical behavior of metallic nanowires within photonic crystal fibers, carrying broad-ranging applications in photonics and nanotechnology. Looking forward, there lies a fertile ground for future exploration in optimizing these structures for diverse applications, including improved sensor designs, microfluidic devices for biochemical sensing, and integration into broader optical systems for telecommunications.

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