Origin of heart-shaped intra-cycle temporal-shift interference patterns in RESI with few-cycle pulses

Determine the physical origin and mechanism of the heart-shaped interference structures that appear in intra-cycle temporal-shift interference maps for recollision-excitation with subsequent ionization (RESI) driven by few-cycle sin^2 pulses. Specifically, derive analytic conditions connecting these shapes to the temporal-shift phase-difference components—α^(A^2)_{Δτ}(t',t''), α^(pond)_{Δτ}(t,t''), α^(ene)_{Δτ}, and α^{(p1,p2)}_{Δτ}(t,t')—and identify the carrier-envelope phase and event-dominance regimes under which these structures emerge or vanish.

Background

In this work, the authors analyze single-channel quantum interference in nonsequential double ionization (NSDI) via the RESI mechanism using few-cycle laser pulses, deriving generalized phase-difference conditions for exchange and event (temporal-shift) interference. They identify multiple field-dependent building blocks for event interference, including terms from the squared vector potential, ponderomotive energy, bound-state and kinetic energies, and momentum–field couplings.

While dissecting interference patterns associated with purely temporal shifts, the authors observe distinctive wing-like and heart-shaped structures in the first or third quadrants (depending on dominant events), alongside static-like patterns in the opposite quadrants. Despite proposing that these heart-shaped patterns likely result from combinations of field-dependent temporal-shift phases, they explicitly state that the origin of this shape is unclear, highlighting a concrete unresolved question about its mechanism and analytic description.

References

In addition to the wings, the intracycle shifts also exhibit heart shapes in the first or third quadrants (depending on the dominance of events involved), with 'static' like patterns in the opposing quadrant. In panel (d) the heart disappears, presumably because for CEP 155°, p3o4 loses dominance. The origin of this shape is unclear. However, this behavior indicates that they may arise from a combination of the field-dependent temporal-shift phase differences.

Detangling the quantum tapestry of intra-channel interference in below-threshold nonsequential double ionization with few-cycle laser pulses  (2404.01056 - Hashim et al., 2024) in Section 5.2 (Event Interference), discussion of Fig. 18