Indirect Excitons and Many-body Interactions in InGaAs Double Quantum Wells (2504.01155v1)

Abstract: Spatially indirect excitons in semiconductor quantum wells are relevant to basic research and device applications because they exhibit enhanced tunability, delocalized wave functions, and potentially longer lifetimes relative to direct excitons. Here we investigate the properties of indirect excitons and their coupling interactions with direct excitons in asymmetric InGaAs double quantum wells using optical multidimensional coherent spectroscopy and photoluminescence excitation spectroscopy. Analyses of the spectra confirm a strong influence of many-body effects, and reveal that excited-state zero-quantum coherences between direct and indirect excitons in the quantum wells dephase faster than the much higher-energy single-quantum coherences between excitonic excited states and ground states. The results also suggest an important energy-dependent role of continuum states in mediating system dynamics, and they indicate that dephasing mechanisms are associated with uncorrelated or anticorrelated energy-level fluctuations.