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Photoacoustic phase-controlled Fourier-transform infrared spectroscopy (2212.10084v1)

Published 20 Dec 2022 in physics.optics, physics.chem-ph, and physics.ins-det

Abstract: We demonstrate a 13-fold speed improvement in broadband cantilever-enhanced photoacoustic spectroscopy (CEPAS) by combining it with phase-controlled Fourier-transform spectroscopy (PC-FTS) instead of traditional Fourier-transform infrared spectroscopy (FTIR). PC-FTS is a modification of FTIR and capable of fundamentally faster interferogram acquisitions. The speed-improvement is beneficial for CEPAS, which is an especially sensitive version of the background-free photoacoustic spectroscopy technique. We used the PC-FTS-CEPAS technique to measure the absorption spectrum of methane in the mid-infrared region (3.3$-$3.5 $\mu$m) with an optical frequency comb as the light source.

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