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Self-attractive semiflexible polymers under an external force field (2211.01274v1)

Published 2 Nov 2022 in cond-mat.soft

Abstract: The dynamical response of a tethered semiflexible polymer with self-attractive interactions and subjected to an external force field is numerically investigated by varying stiffness and self-interaction strength. The chain is confined in two spatial dimensions and placed in contact with a heat bath described by the Brownian multiparticle collision method. For strong self-attraction the equilibrium conformations range from compact structures to double-stranded chains, and to rods when increasing the stiffness. Under the external field at small rigidities, the initial close-packed chain is continuously unwound by the force before being completely elongated. For double-stranded conformations the transition from the folded state to the open one is sharp being steeper for larger stiffnesses. The discontinuity in the transition appears in the force-extension relation as well as in the probability distribution function of the gyration radius. The relative deformation with respect to the equilibrium case along the direction normal to the force is found to decay as the inverse of the applied force.

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