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Quantum Nonlinear Optics with a Germanium-Vacancy Color Center in a Nanoscale Diamond Waveguide (1612.03036v3)

Published 9 Dec 2016 in quant-ph, cond-mat.mes-hall, and physics.optics

Abstract: We demonstrate a quantum nanophotonics platform based on germanium-vacancy (GeV) color centers in fiber-coupled diamond nanophotonic waveguides. We show that GeV optical transitions have a high quantum efficiency and are nearly lifetime-broadened in such nanophotonic structures. These properties yield an efficient interface between waveguide photons and a single GeV without the use of a cavity or slow-light waveguide. As a result, a single GeV center reduces waveguide transmission by $18 \pm 1\%$ on resonance in a single pass. We use a nanophotonic interferometer to perform homodyne detection of GeV resonance fluorescence. By probing the photon statistics of the output field, we demonstrate that the GeV-waveguide system is nonlinear at the single-photon level.

Citations (223)

Summary

  • The paper demonstrates efficient photon-atom coupling where a single GeV center modulates waveguide transmission by 18%.
  • It uses resonant optical excitation achieving near-lifetime-limited linewidths, indicating coherent control in a nanophotonic environment.
  • The study highlights potential for scalable, room-temperature quantum optical networks via robust GeV center interactions.

Quantum Nonlinear Optics with Germanium-Vacancy Centers in Diamond Waveguides

The paper explores the use of germanium-vacancy (GeV) color centers in nanophotonic diamond waveguides as a promising platform for quantum nonlinear optics. The paper's core focus is the demonstration of efficient coupling between single GeV centers and waveguide photons, achieved without the necessity of complex photonic structures like cavities. This represents a crucial step forward for integrated quantum optical networks.

The GeV centers, a relatively new addition to the family of diamond color centers, exhibit favorable optical properties, including high quantum efficiency and minimal spectral broadening. The unique electronic structure of the GeV center, with a spin-doublet ground state and a four-level optical transition system, facilitates effective manipulation of the system using optical and microwave fields. These characteristics are harnessed in the paper to construct a photonics platform where a single GeV center significantly modulates waveguide transmission by 18%, underscoring a strong photon-atom interaction.

The paper provides a comprehensive examination of the GeV center integrated into waveguide devices, highlighting the high radiative quantum efficiency and significant modulation of waveguide transmission. Through resonant optical excitation, the researchers achieve near-lifetime-limited linewidths for the GeV optical transitions, even in the nanophotonic environment. Such efficient interactions are essential for practical implementations of quantum networks and quantum nonlinear optics at the few-photon level.

Key experimental observations include optical Rabi oscillations of the GeV center, indicating coherent control over the optical transitions, and evidence of a high sensitivity to changes in the photonic environment. The paper also shows that the optical coherence of the GeV center is robust up to elevated temperatures, which can be advantageous for room-temperature quantum devices. The measured cooperativity indicates the potential for substantial photon-atom interaction strengths, enabling significant modulation of transmitted light.

One of the notable outcomes of the paper is the demonstration of quantum nonlinearity at the single-photon level through photon statistics analysis. This was achieved through a homodyne interferometer setup, verifying that a single GeV can alter the photon statistics of an output field, a haLLMark of quantum nonlinear optical behavior.

Theoretical implications from these findings suggest promising paths for integrated quantum photonics applications. The demonstrated strengths of the GeV center in nanophotonic waveguides could lead to the development of scalable quantum networks featuring robust, high-coherence spin-photon interfaces. Such interfaces are integral for quantum communication and computation, where they could be used to create quantum nodes with strong atom-light coupling, capable of processing quantum information efficiently and effectively.

Future work will likely focus on optimizing the spin coherence properties of GeV centers, perhaps through low-temperature operations, while leveraging the measured high quantum efficiency for improved photon emission into waveguide modes. Moreover, integration with advanced photonic structures could enhance cooperativity further, potentially enabling deterministic single-photon switching and interactions—a critical capability for advancing quantum optical computing and communication technologies.

In conclusion, the paper effectively establishes germanium-vacancy centers in diamond waveguides as a powerful platform for quantum optics, paving the way for future developments in manipulating and interfacing quantum states within integrated photonic systems.

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