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Correlated-Disordered Metasurfaces

Updated 7 July 2026
  • Correlated-disordered metasurfaces are planar arrays that use intentional spatial correlations, exclusion rules, and hyperuniform patterns to tailor optical responses.
  • They employ controlled displacement and topological descriptors to tune key attributes like specular reflection, resonant linewidths, and far-field scattering.
  • Advanced metrics, including persistent homology and reciprocal-space analysis, enable inverse design and predictive modeling of complex electromagnetic interactions.

Correlated-disordered metasurfaces are planar assemblies of meta-atoms or scatterers that lack global periodicity but retain engineered spatial correlations, so that pair separations, local exclusion rules, reciprocal-space constraints, or connectivity statistics become design variables rather than fabrication byproducts. In this setting, disorder is not restricted to Poisson-like randomness: it can be imposed through minimum inter-particle distances, Gaussian-correlated lattice perturbations, hyperuniform or stealthy-hyperuniform point patterns, shuffled lattices, or connected morphologies near a critical packing threshold. Across these realizations, correlated disorder is used to control specular and diffuse scattering, collective resonances, photon density of states, localization, directional emission, broadband absorption, and visual appearance in ways that are not accessible with either perfect periodicity or purely uncorrelated disorder (Madeleine et al., 2023, Lalanne et al., 2023).

1. Definitions, disorder classes, and structural control

A central distinction is between uncorrelated and correlated positional disorder. In perturbed lattices, uncorrelated disorder is generated by independently displacing each lattice site by a random vector, whereas correlated disorder introduces spatial smoothing so that nearby sites move coherently (Madeleine et al., 2023). In one generative model for metasurfaces of pitch PP, each nanostructure at position ri\mathbf r_i is displaced by Δri\Delta \mathbf r_i with components uniformly drawn in [SdP,SdP][-S_d P, S_d P], and correlations are added through a Gaussian weight

Cij=exp ⁣{[rij2LcP]2},C_{ij}=\exp\!\left\{-\left[\frac{r_{ij}}{2L_cP}\right]^2\right\},

with full width at half maximum 22ln2LcP2\sqrt{2\ln 2}\,L_cP, so that the total perturbation is

ri=ri+Δri+jiΔrjCij.\mathbf r_i'=\mathbf r_i+\Delta \mathbf r_i+\sum_{j\neq i}\Delta \mathbf r_j\,C_{ij}.

Here SdS_d controls displacement amplitude and LcL_c the correlation length and smoothness of the distortion (Madeleine et al., 2023).

A second broad class arises from exclusion constraints. Random sequential addition, Poisson-disk sampling, and related hard-core processes enforce a minimum spacing and therefore generate short-range repulsion and short-range order rather than independent point placement. In the optics literature this correlated-disorder class is frequently used to suppress diffuse scattering near the specular direction or to regularize fabrication-robust layouts (Vynck et al., 2022, Lalanne et al., 2023). In shuffled lattices, such as randomly jittered silicon nanopillar arrays of nominal period P0=310nmP_0=310\,\mathrm{nm}, short-range positional correlations remain centered around the original lattice spacing while long-range order and Bragg peaks are progressively smeared as the disorder parameter increases; at large jitter, close, far, and even overlapping arrangements can occur because no strict hard-core exclusion is imposed (Chen et al., 16 Mar 2025).

Hyperuniform and stealthy-hyperuniform patterns constitute a reciprocal-space definition of correlated disorder. With mean density ri\mathbf r_i0, pair correlation ri\mathbf r_i1, and ri\mathbf r_i2, the static structure factor is

ri\mathbf r_i3

Hyperuniformity requires ri\mathbf r_i4, equivalently a number variance scaling slower than Poisson, while stealthy hyperuniformity imposes ri\mathbf r_i5 for ri\mathbf r_i6 (Madeleine et al., 2023, Monsarrat et al., 2021, Castro-Lopez et al., 2017). In metasurface design this suppresses long-wavelength density fluctuations and concentrates scattering into selected momentum channels.

A further structural regime appears when the notion of isolated meta-atoms begins to break down. In ultrathin dielectric metasurfaces patterned from square posts, a “critical packing regime” occurs when a significant fraction of metaatoms become physically connected; in the reported scanning electron micrographs this corresponds to about half of the metaatoms touching, with short chains and loops coexisting with isolated posts (Chen et al., 4 May 2025). This regime is neither a dilute particulate topology nor a fully semi-continuous aggregate, and its optical response cannot be reduced to either limit.

2. Structural descriptors beyond conventional disorder parameters

For metasurfaces with weak or uncorrelated positional disorder, conventional descriptors such as ri\mathbf r_i7, nearest-neighbor distributions, and Fourier-based metrics are often sufficient. Under strong correlations, however, these descriptors become less reliable as universal disorder coordinates. In strongly correlated Gaussian-distorted lattices, collective point displacements obscure the original lattice, broaden the accessible configuration space, and make the generative parameter ri\mathbf r_i8 a poor proxy for “how disordered” a sample actually is; finite-size windows and measurement noise further degrade statistical descriptors (Madeleine et al., 2023).

A topology-inspired alternative uses persistent homology on the point coordinates. A Vietoris–Rips filtration is built by drawing balls of radius ri\mathbf r_i9, connecting points whose balls intersect, and tracking topological features as Δri\Delta \mathbf r_i0 grows. In two dimensions, the main features are connected components Δri\Delta \mathbf r_i1 and loops Δri\Delta \mathbf r_i2, summarized by Betti numbers Δri\Delta \mathbf r_i3 and Δri\Delta \mathbf r_i4 as functions of Δri\Delta \mathbf r_i5, or by the birth–death pairs Δri\Delta \mathbf r_i6 forming a persistence diagram Δri\Delta \mathbf r_i7 (Madeleine et al., 2023). On this basis, two disorder descriptors were introduced:

Δri\Delta \mathbf r_i8

and

Δri\Delta \mathbf r_i9

with [SdP,SdP][-S_d P, S_d P]0 and [SdP,SdP][-S_d P, S_d P]1 the number of [SdP,SdP][-S_d P, S_d P]2 features. In the reported interpretation, [SdP,SdP][-S_d P, S_d P]3 is a proxy for the typical nearest-neighbor scale, whereas [SdP,SdP][-S_d P, S_d P]4 is minimal for ordered lattices, invariant under global rescaling, independent of dataset size [SdP,SdP][-S_d P, S_d P]5, and orthogonal to [SdP,SdP][-S_d P, S_d P]6 (Madeleine et al., 2023).

The computational pipeline used these descriptors on 1203 perturbed square-lattice patterns with [SdP,SdP][-S_d P, S_d P]7, [SdP,SdP][-S_d P, S_d P]8, and [SdP,SdP][-S_d P, S_d P]9, each containing Cij=exp ⁣{[rij2LcP]2},C_{ij}=\exp\!\left\{-\left[\frac{r_{ij}}{2L_cP}\right]^2\right\},0 points. Vietoris–Rips filtrations were computed with Ripser; Wasserstein distances between persistence diagrams were computed with GUDHI and embedded by classical multidimensional scaling. The reported behavior was that uncorrelated disorder yielded clear clustering by Cij=exp ⁣{[rij2LcP]2},C_{ij}=\exp\!\left\{-\left[\frac{r_{ij}}{2L_cP}\right]^2\right\},1, intermediate correlation widened and overlapped clusters, and strong correlation merged them, making the generative parameters unreliable predictors. Coloring the same embeddings by Cij=exp ⁣{[rij2LcP]2},C_{ij}=\exp\!\left\{-\left[\frac{r_{ij}}{2L_cP}\right]^2\right\},2 recovered the spacing scale across Cij=exp ⁣{[rij2LcP]2},C_{ij}=\exp\!\left\{-\left[\frac{r_{ij}}{2L_cP}\right]^2\right\},3, while coloring by Cij=exp ⁣{[rij2LcP]2},C_{ij}=\exp\!\left\{-\left[\frac{r_{ij}}{2L_cP}\right]^2\right\},4 recovered disorder strength across Cij=exp ⁣{[rij2LcP]2},C_{ij}=\exp\!\left\{-\left[\frac{r_{ij}}{2L_cP}\right]^2\right\},5 and Cij=exp ⁣{[rij2LcP]2},C_{ij}=\exp\!\left\{-\left[\frac{r_{ij}}{2L_cP}\right]^2\right\},6 (Madeleine et al., 2023).

Topological descriptors are not the only nontrivial structural measures in the field. In morphogenetically generated correlated media, a translational order metric

Cij=exp ⁣{[rij2LcP]2},C_{ij}=\exp\!\left\{-\left[\frac{r_{ij}}{2L_cP}\right]^2\right\},7

was used to follow the evolution from correlated disorder to crystallization. The reported normalized values were Cij=exp ⁣{[rij2LcP]2},C_{ij}=\exp\!\left\{-\left[\frac{r_{ij}}{2L_cP}\right]^2\right\},8 for early correlated disorder, Cij=exp ⁣{[rij2LcP]2},C_{ij}=\exp\!\left\{-\left[\frac{r_{ij}}{2L_cP}\right]^2\right\},9 for a transitional regime, and 22ln2LcP2\sqrt{2\ln 2}\,L_cP0 for a hexagonal crystal (Chehami et al., 2023). The broader methodological implication is that correlated-disordered metasurfaces are often better characterized by descriptors that remain reference-free under changes of pitch, correlation length, or morphology than by a single generative disorder amplitude.

3. Scattering theory, collective electrodynamics, and reciprocity-space design

The electromagnetic response of disordered metasurfaces is commonly decomposed into coherent and diffuse contributions. For the scattered field,

22ln2LcP2\sqrt{2\ln 2}\,L_cP1

and the averaged intensity separates as

22ln2LcP2\sqrt{2\ln 2}\,L_cP2

Within an independent scattering approximation, the radiant intensity is often written as a single-particle form factor multiplied by a structure factor, while effective-field and quasi-crystalline closures incorporate collective interactions more self-consistently (Vynck et al., 2022, Lalanne et al., 2023). For coherent specular reflection and transmission by a particle monolayer, the analytical expressions in the independent scattering approximation and the effective field approximation depend explicitly on the one-point density and the single-particle scattering amplitude; pair correlations enter the coherent channel only through more advanced closures such as QCA or through full-wave simulations (Vynck et al., 2022).

In dense or resonant metasurfaces, discrete-element electrodynamics becomes essential. For asymmetrically split-ring arrays, each resonant arc is modeled as a damped oscillator and all recurrent scattering processes are retained through a many-body coupling matrix 22ln2LcP2\sqrt{2\ln 2}\,L_cP3, so that the collective amplitudes obey

22ln2LcP2\sqrt{2\ln 2}\,L_cP4

with collective eigenvalues

22ln2LcP2\sqrt{2\ln 2}\,L_cP5

This microscopic description captures radiative and non-radiative decay, retardation, electric–electric and magnetic–magnetic dipole interactions, and electric–magnetic cross-coupling (Jenkins et al., 2018). The central physical point is that the response of a disordered metasurface is mapped from pair separations and multiple scattering sequences into collective linewidths, frequency shifts, mode localization, and far-field resonances.

For arrays supporting surface lattice resonances, periodic references remain useful. In a square lattice of pitch 22ln2LcP2\sqrt{2\ln 2}\,L_cP6 and effective refractive index 22ln2LcP2\sqrt{2\ln 2}\,L_cP7, the Rayleigh anomaly for diffraction order 22ln2LcP2\sqrt{2\ln 2}\,L_cP8 satisfies

22ln2LcP2\sqrt{2\ln 2}\,L_cP9

Correlated disorder can emulate effective lattice vectors through short-range order and peaks in ri=ri+Δri+jiΔrjCij.\mathbf r_i'=\mathbf r_i+\Delta \mathbf r_i+\sum_{j\neq i}\Delta \mathbf r_j\,C_{ij}.0, thereby supporting SLR-like diffractive coupling without perfect periodicity (Madeleine et al., 2023).

A distinct analytical framework emerges when disorder itself is designed in reciprocal space. For lattices perturbed by correlated random displacements, the disorder statistics define three scattering components: a diffuse background, Bragg-like diffraction orders, and correlation halos. The halo term is absent for uncorrelated disorder, depends on the increment distributions ri=ri+Δri+jiΔrjCij.\mathbf r_i'=\mathbf r_i+\Delta \mathbf r_i+\sum_{j\neq i}\Delta \mathbf r_j\,C_{ij}.1, and can be positive or negative. In consequence, correlation halos are not broadened diffraction peaks; they are independent features whose positions depend on the correlation range and can remain visible after ordinary diffraction orders vanish (Langevin et al., 19 Feb 2026). This result expands the standard view in which disorder merely broadens reciprocal-lattice peaks into a broadband background.

4. Resonances, localization, and experimentally observed optical regimes

The reported optical consequences of correlated disorder are diverse because the relevant mechanisms differ across metasurface classes. In plasmonic nanoparticle lattices designed with topological descriptors, the strength of surface lattice resonances was correlated with ri=ri+Δri+jiΔrjCij.\mathbf r_i'=\mathbf r_i+\Delta \mathbf r_i+\sum_{j\neq i}\Delta \mathbf r_j\,C_{ij}.2 while keeping ri=ri+Δri+jiΔrjCij.\mathbf r_i'=\mathbf r_i+\Delta \mathbf r_i+\sum_{j\neq i}\Delta \mathbf r_j\,C_{ij}.3 approximately fixed. In theory, for gold nanocylinders of height ri=ri+Δri+jiΔrjCij.\mathbf r_i'=\mathbf r_i+\Delta \mathbf r_i+\sum_{j\neq i}\Delta \mathbf r_j\,C_{ij}.4 and diameter ri=ri+Δri+jiΔrjCij.\mathbf r_i'=\mathbf r_i+\Delta \mathbf r_i+\sum_{j\neq i}\Delta \mathbf r_j\,C_{ij}.5 in a medium of refractive index ri=ri+Δri+jiΔrjCij.\mathbf r_i'=\mathbf r_i+\Delta \mathbf r_i+\sum_{j\neq i}\Delta \mathbf r_j\,C_{ij}.6, three metasurfaces selected at the same ri=ri+Δri+jiΔrjCij.\mathbf r_i'=\mathbf r_i+\Delta \mathbf r_i+\sum_{j\neq i}\Delta \mathbf r_j\,C_{ij}.7 but different ri=ri+Δri+jiΔrjCij.\mathbf r_i'=\mathbf r_i+\Delta \mathbf r_i+\sum_{j\neq i}\Delta \mathbf r_j\,C_{ij}.8 showed progressively weaker resonances as ri=ri+Δri+jiΔrjCij.\mathbf r_i'=\mathbf r_i+\Delta \mathbf r_i+\sum_{j\neq i}\Delta \mathbf r_j\,C_{ij}.9 increased, with reported quality factors SdS_d0, SdS_d1, and SdS_d2 from lowest to highest SdS_d3. In experiment, focused-ion-beam-fabricated elongated gold nanodisks coated with IC1-200 and measured at normal incidence showed that in 5 out of 6 correlated comparisons the metasurface with lower SdS_d4, even when SdS_d5 was larger, exhibited higher SdS_d6 (Madeleine et al., 2023).

Pattern TD Reported SdS_d7
periodic, SdS_d8 0.000 10.1, 11.5
SdS_d9 0.030 4.0, 5.2
LcL_c0 0.012 9.3, 6.8
LcL_c1 0.025 6.7, 4.4
LcL_c2 0.005 7.8, 7.0
LcL_c3 0.026 8.0, 11.5
LcL_c4 0.002 10.1, 11.5

The main exception occurred for LcL_c5 and perpendicular polarization, where both correlated samples had LcL_c6 because large LcL_c7 smooths short-range disorder while preserving long-scale distortions; LcL_c8 detects the latter, whereas SLRs remain robust to it (Madeleine et al., 2023).

In metamaterial arrays with strong radiative interactions, positional disorder drives a different transition. In a regular LcL_c9 array of asymmetrically split rings, approximately P0=310nmP_0=310\,\mathrm{nm}0 of the driven response concentrates into a single spatially extended many-body subradiant eigenmode with magnetic dipoles in phase and collective decay rate P0=310nmP_0=310\,\mathrm{nm}1. A gradual increase of positional disorder rapidly localizes the mode and red-shifts the far-field transmission resonance through a cooperative Lamb shift; for one representative realization, P0=310nmP_0=310\,\mathrm{nm}2 increased only weakly to P0=310nmP_0=310\,\mathrm{nm}3 at P0=310nmP_0=310\,\mathrm{nm}4, showing that localization and subradiance can coexist at moderate disorder (Jenkins et al., 2018).

Correlated disorder also modifies the density of states and localization in two-dimensional resonant media. For vector TE waves in stealth-hyperuniform point patterns, localization occurs at moderate density in the same window where the density of states exhibits a pseudo-gap; the reported localization island appears around P0=310nmP_0=310\,\mathrm{nm}5–P0=310nmP_0=310\,\mathrm{nm}6 and P0=310nmP_0=310\,\mathrm{nm}7, whereas no signature of localization is found for white-noise disorder. For scalar TM waves, localization occurs at high density irrespective of correlations (Monsarrat et al., 2021). The proposed microscopic origin is destructive interference between independent scattering and recurrent loop scattering weighted by the short-range peak of P0=310nmP_0=310\,\mathrm{nm}8 near P0=310nmP_0=310\,\mathrm{nm}9.

Near the critical packing threshold, connected dielectric metasurfaces display abrupt far-field changes tied to a redistribution of quasi-normal modes in the complex-frequency plane. In particulate arrays, the photon density of states contains clustered clouds and bandgap-like voids; at critical packing these voids begin to vanish and new collective resonances shift to lower frequencies; in aggregate regimes the PDoS becomes broad and nearly uniform across the visible, with ri\mathbf r_i00 factors generally below ri\mathbf r_i01 (Chen et al., 4 May 2025). In the far field, correlated particulate arrays show a blue shift of the diffuse BRDF maximum with increasing density, while transitions into critical and aggregate regimes produce broadband diffuse whitening. For ri\mathbf r_i02, ri\mathbf r_i03, and ri\mathbf r_i04, the reported diffuse brightness approaches ri\mathbf r_i05 across the visible even though the structure is a single ri\mathbf r_i06 poly-Si layer, and at critical packing a broadband specular “mirror” peak reaches ri\mathbf r_i07 near ri\mathbf r_i08 with ri\mathbf r_i09 (Chen et al., 4 May 2025).

Hyperuniform reciprocal-space engineering leads to yet another regime: isotropic annular scattering and emission. Gold metasurfaces derived from stealth-hyperuniform point sets with stealthiness ri\mathbf r_i10 and 4000 points exhibit a single broad isotropic diffraction maximum, and both scattering and fluorescence measurements show rotationally symmetric rings at in-plane momentum

ri\mathbf r_i11

so that ri\mathbf r_i12. The opening of the ring therefore scales with the inverse correlation length parameter ri\mathbf r_i13, and in fluorescence the ring closes near ri\mathbf r_i14 because of band folding into the light cone (Castro-Lopez et al., 2017).

A separate application to infrared silicon photodetection uses a shuffled-lattice disordered metasurface integrated with upconversion nanoparticles. In that work the layout is generated by independent uniform jitter of Si nanopillars around a square lattice, and the paper does not report explicit correlation descriptors such as ri\mathbf r_i15 or ri\mathbf r_i16; nevertheless, the highly disordered configuration with ri\mathbf r_i17 is reported to increase infrared absorption by ri\mathbf r_i18-fold and the near field by ri\mathbf r_i19-fold relative to the ordered structure, while the measured responsivity at ri\mathbf r_i20 reaches ri\mathbf r_i21 at room temperature, corresponding to an external quantum efficiency of ri\mathbf r_i22 (Chen et al., 16 Mar 2025). The stated mechanism is disorder-induced mode packing of hybrid Mie–plasmonic cavities together with field enhancement that boosts Erri\mathbf r_i23 upconversion and hot-electron generation.

5. Design methodologies, fabrication routes, and inverse design

A practical design workflow for correlated-disordered metasurfaces has been articulated most explicitly for topological learning. The sequence is: specify a target optical property, choose a disorder model such as minimum-distance-constrained patterns, Gaussian-correlated displacements, or hyperuniform and stealthy-hyperuniform patterns, generate candidate point sets over ranges of ri\mathbf r_i24, ri\mathbf r_i25, pitch, or minimum spacing, compute Vietoris–Rips persistence diagrams and the descriptors ri\mathbf r_i26 and ri\mathbf r_i27, select patterns at matched ri\mathbf r_i28 and desired ri\mathbf r_i29, predict the optical response with a dipole approximation or a learned regression, and then iterate until the target metrics are met before fabrication and validation (Madeleine et al., 2023). In this formulation, ri\mathbf r_i30 fixes local spacing while ri\mathbf r_i31 ranks positional disorder.

Morphogenetic design provides a different route to correlated disorder by replacing global optimization with local reaction–diffusion rules. In the Gray–Scott model,

ri\mathbf r_i32

the reported parameter set ri\mathbf r_i33, ri\mathbf r_i34, ri\mathbf r_i35, ri\mathbf r_i36 generates self-replicating spots whose early-time patterns are stealthy-hyperuniform-like and isotropic in ri\mathbf r_i37, whose transitional states develop weak local crystallites, and whose late-time states converge toward a compact hexagonal crystal (Chehami et al., 2023). After thresholding at ri\mathbf r_i38, the reported supercells yield spot diameters of about ri\mathbf r_i39 and average center-to-center spacing of about ri\mathbf r_i40. Extruded into dielectric rods of ri\mathbf r_i41 in air, these patterns produce isotropic microwave TM bandgaps with reported normalized widths of approximately ri\mathbf r_i42 in the correlated-disordered state, ri\mathbf r_i43 in the transitional state, and ri\mathbf r_i44 in the crystal (Chehami et al., 2023). The method is notable because the paper states that it eliminates cost-function minimization and is natively scalable to large domains.

Reciprocal-space engineering begins from a target ri\mathbf r_i45 rather than a real-space motif. In hyperuniform gold metasurfaces, a point pattern was chosen so that ri\mathbf r_i46 had a pronounced exclusion region near ri\mathbf r_i47 and a single broad isotropic maximum at ri\mathbf r_i48; pillar-type and network-type layouts were then produced while preserving the dominant isotropic resonance (Castro-Lopez et al., 2017). In a more general correlated-noise framework, the averaged far-field intensity is expressed as the sum of a diffuse term, a Bragg term, and a correlation-halo term, with the displacement probability density function ri\mathbf r_i49 and the correlation length ri\mathbf r_i50 as independent design knobs. The paper gives an explicit constructive example,

ri\mathbf r_i51

whose Fourier transform preserves only selected diffraction orders; for ri\mathbf r_i52, the retained orders are ri\mathbf r_i53 with reported intensities ri\mathbf r_i54 at specular and ri\mathbf r_i55 at ri\mathbf r_i56 (Langevin et al., 19 Feb 2026). The same paper describes the resulting framework as a practical method for inverse design, namely finding the disorder that produces desired scattering patterns.

Fabrication routes reflect the breadth of the field. Reported examples include focused-ion-beam fabrication of gold nanodisks on ri\mathbf r_i57 areas followed by spin-coating with IC1-200 (Madeleine et al., 2023), electron-beam lithography and reactive-ion etching of ri\mathbf r_i58 poly-Si on fused silica with tunable connectivity (Chen et al., 4 May 2025), electron-beam lithography and ICP etching of Si nanopillars followed by ri\mathbf r_i59 Al deposition and spin-coated NaYFri\mathbf r_i60:Erri\mathbf r_i61 core–shell nanoparticles (Chen et al., 16 Mar 2025), electron-beam lithography of hyperuniform gold pillars and networks on glass followed by a ri\mathbf r_i62 PMMA layer doped with DCM dye (Castro-Lopez et al., 2017), and colloidal deposition of approximately ri\mathbf r_i63 silver nanocubes above a SiOri\mathbf r_i64/Si reflector (Agreda et al., 2022). Large-area and bottom-up routes are likewise emphasized in the broader review literature because correlated disorder can be more fabrication-resilient than tightly periodic phase profiles (Lalanne et al., 2023).

6. Misconceptions, limitations, and research directions

A recurrent misconception is that disorder in metasurfaces is synonymous with uncontrollable whitish diffuse scattering. Several results contradict that reduction. Correlated disorder can support sharp or quasi-sharp collective resonances, isotropic momentum-space rings, specular suppression near ri\mathbf r_i65, critical-packing mirror peaks, prescribed diffuse whitening, or Morpho-like correlation halos (Madeleine et al., 2023, Castro-Lopez et al., 2017, Chen et al., 4 May 2025, Langevin et al., 19 Feb 2026). Another misconception is that a single scalar disorder amplitude is always a sufficient disorder coordinate. Under strong positional correlations, ri\mathbf r_i66 can become ambiguous, and topological descriptors or reciprocal-space statistics become more informative than the generative parameter itself (Madeleine et al., 2023).

Model validity is strongly regime-dependent. In coherent specular theory, ISA is accurate for very dilute monolayers, and EFA remains quantitatively useful up to about ri\mathbf r_i67 coverage and large angles for high-index dielectric particles, but for plasmonic particles at comparable coverage strong near-field coupling and hot spots degrade both approximations (Vynck et al., 2022). In critical-packing dielectric metasurfaces, extended Maxwell–Garnett modeling matches particulate regimes but underestimates the strong reflection peak near the connectivity threshold because connected-cluster physics and collective electric–magnetic dipolar response are not captured by a local effective medium (Chen et al., 4 May 2025). In SLR design, global ri\mathbf r_i68 can overestimate disorder that does not materially affect the resonance quality factor because long-scale distortions matter less than short-range coupling; a local ri\mathbf r_i69 computed in sliding windows was proposed as a better match to near-field interaction ranges (Madeleine et al., 2023).

The physical role of correlations is also not monotonic. Large ri\mathbf r_i70 can improve short-range order and preserve high-ri\mathbf r_i71 resonances even while increasing global topological disorder; hyperuniformity can reduce low-angle scattering and broaden absorption; connected morphologies can whiten diffuse light but also erase spectral selectivity by filling PDoS voids (Madeleine et al., 2023, Chen et al., 4 May 2025). Polarization dependence remains important in several platforms, from elongated plasmonic nanodisks to TE/TM localization windows in resonant point patterns (Madeleine et al., 2023, Monsarrat et al., 2021). In particular, the localization results in correlated two-dimensional media show that vector TE waves localize in a correlated moderate-density regime but exhibit no localization signature in white-noise disorder, whereas scalar TM waves localize at high density regardless of correlation class (Monsarrat et al., 2021).

Current research directions accordingly emphasize descriptors and models that preserve structural universality while remaining tied to physically relevant coupling scales. Reported directions include localized topological descriptors aligned with coupling radii and integration with inverse design, topology optimization, and graph neural networks using topological features as priors or constraints (Madeleine et al., 2023); nonlocal effective models and polarization control for critical-packing topologies (Chen et al., 4 May 2025); and broader k-space design of hyperuniform, quasi-periodic, or multilayer correlated-disordered metasurfaces for broadband antireflection, structural color, transparent displays, chiral films, light trapping, and wavefront manipulation (Lalanne et al., 2023). The field’s unifying idea is that disorder becomes most useful when it is specified statistically, topologically, or in reciprocal space rather than treated as an uncontrolled deviation from a crystal.

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