Evidence of Ultrashort Orbital Transport in Heavy Metals Revealed by Terahertz Emission Spectroscopy (2504.15553v2)

Abstract: The orbital angular momentum of electrons offers a promising, yet largely unexplored, degree of freedom for ultrafast, energy-efficient information processing. As the foundation of orbitronics, understanding how orbital currents propagate and convert into charge currents is essential - but remains elusive due to the challenge in disentangling orbital and spin dynamics in ultrathin films. Although orbital currents have been predicted to propagate over long distances in materials, recent theoretical studies argue that lattice symmetry may constrain their mean free paths (MFPs) to the scale of a single atomic layer. In this work, we provide the first direct experimental evidence for ultrashort orbital MFPs in heavy metals (HMs) - W, Ta, Pt - revealed by femtosecond terahertz emission spectroscopy. This is enabled by sub-nanometer-precision control of thin-film thickness using wedge-shaped HM|Ni heterostructures. By employing a multi-component terahertz-emission model, we quantitatively extract the orbital MFPs, consistently finding them shorter than their spin counterparts. Furthermore, control experiments rule out interfacial orbital-to-charge conversion as the dominant mechanism, confirming that the process is governed by the bulk inverse orbital Hall effect. Our findings resolve a central controversy in orbitronics and provide key insights into orbital transport and conversion mechanisms.