Chiral TeraHertz surface plasmonics
Abstract: Chiral engineering of TeraHertz (THz) light fields and the use of the handedness of light in THz light-matter interactions promise many novel opportunities for advanced sensing and control of matter in this frequency range. Unlike previously explored methods, this is achieved here by leveraging the chiral properties of highly confined THz surface plasmon modes. More specifically, we design ultrasmall surface plasmonic-based THz cavities and THz metasurfaces that display significant and adjustable chiral behavior under modest magnetic fields (B<500mT). For such a prototypical example of non-hermitian and dispersive photonic system, we demonstrate the capacity to magnetic field-tune both the poles and zeros of cavity resonances, the two fundamental parameters governing their resonance properties. Alongside the observed handedness-dependent cavity frequencies, this highlights the remarkable ability to engineer chiral and tunable radiative couplings for THz resonators and metasurfaces. The extensive tunability offered by the surface plasmonic approach paves the way for the development of agile and multifunctional THz metasurfaces as well as the realization of ultrastrong chiral light-matter interactions at low energy in matter with potential far-reaching applications for the design of material properties.
- Optical chirality and its interaction with matter. Physical Review Letters, 104(16):163901, April 2010.
- Electromagnetic chirality: from fundamentals to nontraditional chiroptical phenomena. Light: Science and Applications, 9(1), September 2020.
- Enhanced enantioselectivity in excitation of chiral molecules by superchiral light. Science, 332(6027):333–336, April 2011.
- Chirality of matter shows up via spin excitations. Nature Physics, 8(10):734–738, August 2012.
- Chiral quantum optics. Nature, 541(7638):473–480, jan 2017.
- The added value of small-molecule chirality in technological applications. Nature Reviews Chemistry, 1(6), June 2017.
- Chirality in light–matter interaction. Advanced Materials, 35(34), May 2022.
- Cyriaque Genet. Chiral light–chiral matter interactions: an optical force perspective. ACS Photonics, 9(2):319–332, January 2022.
- Chiral phonons in microcrystals and nanofibrils of biomolecules. Nature Photonics, 16(5):366–373, mar 2022.
- Terahertz circular dichroism spectroscopy of molecular assemblies and nanostructures. Journal of the American Chemical Society, 144(50):22789–22804, dec 2022.
- Coherent terahertz control of antiferromagnetic spin waves. Nature Photonics, 5(1):31–34, nov 2010.
- Chirality selective magnon-phonon hybridization and magnon-induced chiral phonons in a layered zigzag antiferromagnet. Nature Communications, 14(1), jun 2023.
- Truly chiral phonons in α𝛼\alphaitalic_α-HgS. Nature Physics, 19(1):35–39, oct 2022.
- Magnetic control of soft chiral phonons in PbTe. Physical Review Letters, 128(7):075901, feb 2022.
- Observation of floquet-bloch states on the surface of a topological insulator. Science, 342(6157):453–457, October 2013.
- Light-induced anomalous hall effect in graphene. Nature Physics, 16(1):38–41, November 2019.
- Topological floquet engineering of twisted bilayer graphene. Physical Review Research, 1(2):023031, September 2019.
- Cavity quantum electrodynamical chern insulator: Towards light-induced quantized anomalous hall effect in graphene. Physical Review B, 99(23):235156, June 2019.
- Engineering quantum materials with chiral optical cavities. Nature Materials, 20(4):438–442, nov 2020.
- Vacuum anomalous hall effect in gyrotropic cavity. Physical Review B, 104(8):l081408, August 2021.
- Cavity-induced chiral edge currents and spontaneous magnetization in two-dimensional electron systems. Physical Review B, 106(20):205114, nov 2022.
- Chiral cavity quantum electrodynamics. Nature Physics, 18(9):1048–1052, jul 2022.
- Berry phase and topology in ultrastrongly coupled quantum light-matter systems. Physical Review B, 107(19):195104, May 2023.
- Photon condensation, van vleck paramagnetism, and chiral cavities. Physical Review Research, 6(1):013303, March 2024.
- Terahertz chiral metamaterial cavities breaking time-reversal symmetry. arXiv.2308.03195, 2023.
- Photoinduced handedness switching in terahertz chiral metamolecules. Nature Communications, 3(1), jul 2012.
- Chiral metafoils for terahertz broadband high-contrast flexible circular polarizers. Physical Review Applied, 2(1):014005, July 2014.
- Enantiomeric switching of chiral metamaterial for terahertz polarization modulation employing vertically deformable MEMS spirals. Nature Communications, 6(1), oct 2015.
- Electrical access to critical coupling of circularly polarized waves in graphene chiral metamaterials. Science Advances, 3(9), September 2017.
- Terahertz circular dichroism spectroscopy of biomaterials enabled by kirigami polarization modulators. Nature Materials, 18(8):820–826, jul 2019.
- Electrically programmable terahertz diatomic metamolecules for chiral optical control. Research, 2019:1–11, February 2019.
- Tunable magneto-optical polarization device for terahertz waves based on insb and its plasmonic structure. Photonics Research, 7(3):325, February 2019.
- Linear-polarized terahertz isolator by breaking the gyro-mirror symmetry in cascaded magneto-optical metagrating. Nanophotonics, 10(16):4141–4148, October 2021.
- Creating a near-perfect circularly polarized terahertz beam through the nonreciprocity of a magnetoplasma. Optics Express, 31(23):38540, October 2023.
- Infrared and microwave magnetoplasma effects in semiconductors. Reports on Progress in Physics, 33(3):1193–1322, September 1970.
- Interference-induced terahertz transparency in a semiconductor magneto-plasma. Nature Physics, 6(2):126–130, December 2009.
- Terahertz frequency hall measurement by magneto-optical kerr spectroscopy in inas. Applied Physics Letters, 81(2):199–201, July 2002.
- Circuit-tunable sub-wavelength thz resonators: hybridizing optical cavities and loop antennas. Optics Express, 22(18):21302, August 2014.
- Few-electron ultrastrong light-matter coupling at 300 ghz with nanogap hybrid lc microcavities. Nano Letters, 17(12):7410–7415, November 2017.
- Nanoscale electromagnetic confinement in thz circuit resonators. Optics Express, 25(23):28718, November 2017.
- Ultrasmall and tunable terahertz surface plasmon cavities at the ultimate plasmonic limit. Nature Communications, 14(1), November 2023.
- Resonant cavity modes of circular plasmonic patch nanoantennas. Applied Physics Letters, 104(2):021111, jan 2014.
- Temporal coupled-mode theory for the fano resonance in optical resonators. Journal of the Optical Society of America A, 20(3):569, March 2003.
- Optical critical coupling into highly confining metal-insulator-metal resonators. Applied Physics Letters, 103(9), August 2013.
- Tailor the functionalities of metasurfaces based on a complete phase diagram. Physical Review Letters, 115(23):235503, December 2015.
- Quasinormal-mode expansion of the scattering matrix. Physical Review X, 7(2):021035, June 2017.
- Quasinormal coupled mode theory. arXiv:2010.08650, 2020.
- Quasi-normal mode theory of the scattering matrix, enforcing fundamental constraints for truncated expansions. Physical Review Research, 3(3):033228, September 2021.
- Theoretical study of the anomalies of coated dielectric gratings. Optica Acta: International Journal of Optics, 33(5):607–619, May 1986.
- Electromagnetic resonances in linear and nonlinear optics: phenomenological study of grating behavior through the poles and zeros of the scattering operator. Journal of the Optical Society of America A, 12(3):513, March 1995.
- Poles and zeros in non-hermitian systems: Application to photonics. Physical Review B, 109(4):045414, January 2024.
- Coherent perfect absorbers: Time-reversed lasers. Physical Review Letters, 105(5):053901, July 2010.
- Time-reversed lasing and interferometric control of absorption. Science, 331(6019):889–892, February 2011.
- Theory of reflectionless scattering modes. Physical Review A, 102(6):063511, December 2020.
- Strong near field enhancement in thz nano-antenna arrays. Scientific Reports, 3(1), March 2013.
- Theory of patch-antenna metamaterial perfect absorbers. Physical Review A, 93(6):063849, June 2016.
- Effective-medium description of a metasurface composed of a periodic array of nanoantennas coupled to a metallic film. Physical Review A, 95(3):033822, March 2017.
- Terahertz chiral metamaterials with giant and dynamically tunable optical activity. Physical Review B, 86(3):035448, jul 2012.
- Formulation for stable and efficient implementation of the rigorous coupled-wave analysis of binary gratings. Journal of the Optical Society of America A, 12(5):1068, May 1995.
- Reticolo software for grating analysis. arXiv:2101.00901, 2021.
- Optical properties of metal-dielectric-metal microcavities in the thz frequency range. Optics Express, 18(13):13886, June 2010.
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