Nonreciprocal directional dichroism induced by a temperature gradient as a probe for mobile spin dynamics in quantum magnets

Abstract: Novel states of matter in quantum magnets like quantum spin liquids attract considerable interest recently. Despite the existence of a plenty of candidate materials, there is no confirmed quantum spin liquid, largely due to the lack of proper experimental probes. For instance, spectrosocopy experiments like neutron scattering receive contributions from disorder-induced local modes, while thermal transport experiments receive contributions from phonons. Here we propose a thermo-optic experiment which directly probes the mobile magnetic excitations in spatial-inversion symmetric and/or time-reversal symmetric Mott insulators: the temperature-gradient-induced nonreciprocal directional dichroism (TNDD) spectroscopy. Unlike traditional probes, TNDD directly detects mobile magnetic excitations and decouples from phonons and local magnetic modes.